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  <doc>
    <id>1611</id>
    <completedYear>2019</completedYear>
    <publishedYear/>
    <thesisYearAccepted/>
    <language>eng</language>
    <pageFirst/>
    <pageLast/>
    <pageNumber/>
    <edition/>
    <issue/>
    <volume/>
    <type>preprint</type>
    <publisherName>Wiley</publisherName>
    <publisherPlace/>
    <creatingCorporation/>
    <contributingCorporation/>
    <belongsToBibliography>0</belongsToBibliography>
    <completedDate>--</completedDate>
    <publishedDate>--</publishedDate>
    <thesisDateAccepted>--</thesisDateAccepted>
    <title language="eng">Building Supramolecular DNA-Inspired Nanowires on Gold Surfaces: From 2D to 3D</title>
    <abstract language="eng">Three building blocks have been designed to chemically link to a gold surface and vertically self-assemble through thymine–adenine hydrogen bonds. Starting from these building blocks, two different films were engineered on gold surface. Film 1 consists of adenine linked to lipoic acid (Lipo–A) to covalently bind to the gold surface, and ZnTPP linked to a thymine (T–ZnTPP). Film 2 has an additional noncovalently linked layer: a helical undecapeptide analogue of the trichogin GA IV peptide, in which four glycines were replaced by four lysines to favor a helical conformation and reduce flexibility and the two extremities were functionalized with thymine and adenine to enable Lipo–A and T–ZnTPP binding, respectively. These films were characterized by electrochemical and spectroscopic techniques, and were very stable over time and when in contact with solution. Under illumination, they could generate current with higher efficiency than similar previously described systems.</abstract>
    <parentTitle language="eng">Angewandte Chemie International Edition</parentTitle>
    <identifier type="urn">urn:nbn:de:kobv:526-opus4-16113</identifier>
    <enrichment key="opus.import.date">2022-05-18T11:16:50+00:00</enrichment>
    <enrichment key="opus.source">sword</enrichment>
    <enrichment key="opus.import.user">sword</enrichment>
    <enrichment key="opus.import.file">filename=phpu9U5BQ</enrichment>
    <enrichment key="opus.import.checksum">8aa146995fd026ab278524f2ecb45300</enrichment>
    <enrichment key="CopyrightInfo">This is the pre-peer reviewed version of the following article: E. Gatto, S. Kubitzky, M. Schriever, S. Cesaroni, C. Mazzuca, G. Marafon, M. Venanzi, M. De Zotti, Angew. Chem. Int. Ed. 2019, 58, 7308., which has been published in final form at https://doi.org/10.1002/anie.201901683. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Use of Self-Archived Versions.</enrichment>
    <enrichment key="DOI_VoR">https://doi.org/10.1002/anie.201901683</enrichment>
    <licence>Das Dokument ist urheberrechtlich geschützt.</licence>
    <author>Emanuela Gatto</author>
    <author>Sascha Kubitzky</author>
    <author>Marc Schriever</author>
    <author>Simona Cesaroni</author>
    <author>Claudia Mazzuca</author>
    <author>Giulia Marafon</author>
    <author>Mariano Venanzi</author>
    <author>Marta De Zotti</author>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>peptide</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>photocurrent generation</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>self-assembled monolayer</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>self-assembly</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>supramolecular chemistry</value>
    </subject>
    <collection role="ddc" number="660">Chemische Verfahrenstechnik</collection>
    <collection role="institutes" number="">Fachbereich Ingenieur- und Naturwissenschaften</collection>
    <collection role="open_access" number="">open_access</collection>
    <collection role="Import" number="import">Import</collection>
    <collection role="green_open_access" number="2">Green Open Access</collection>
    <thesisPublisher>Technische Hochschule Wildau</thesisPublisher>
    <file>https://opus4.kobv.de/opus4-th-wildau/files/1611/201901683.pdf</file>
  </doc>
</export-example>
