<?xml version="1.0" encoding="utf-8"?>
<export-example>
  <doc>
    <id>563</id>
    <completedYear>2000</completedYear>
    <publishedYear>2000</publishedYear>
    <thesisYearAccepted/>
    <language>eng</language>
    <pageFirst>256</pageFirst>
    <pageLast>262</pageLast>
    <pageNumber/>
    <edition/>
    <issue>1-3</issue>
    <volume>318</volume>
    <type>article</type>
    <publisherName/>
    <publisherPlace/>
    <creatingCorporation/>
    <contributingCorporation/>
    <belongsToBibliography>1</belongsToBibliography>
    <completedDate>2014-07-02</completedDate>
    <publishedDate>--</publishedDate>
    <thesisDateAccepted>--</thesisDateAccepted>
    <title language="eng">Ab initio three-dimensional quantum dynamics of Ag3 clusters in the NeNePo process</title>
    <abstract language="eng">The first three-dimensional quantum-dynamical ab initio simulation of the large amplitude vibrational dynamics of an Ag3 cluster initiated from its linear transition state is presented. This can be monitored by femtosecond pump-probe negative-ion to neutral-to-positive-ion spectroscopy with zero electron kinetic energy (NeNePo-ZEKE). The time evolution of the representative wavepacket confirms the dynamical effects which have been discovered previously by Wigner-type semiclassical simulations: the initial coherent bending and stretching from linear to near equilateral triangular configuration, followed by intracluster collision and intracluster vibrational relaxation with a weak fractional revival. In addition, the quantum wavepacket shows interferences and spreading.</abstract>
    <parentTitle language="eng">Chemical Physics Letters</parentTitle>
    <identifier type="urn">urn:nbn:de:0298-opus4-5637</identifier>
    <enrichment key="PeerReviewed">Keine Angabe - No details</enrichment>
    <enrichment key="LinkProfileA">https://www.srh-berlin.de/hochschule/hochschulteam/hartmann-michael/</enrichment>
    <author>Igor Andrianov</author>
    <author>Vlasta Bonačić-Koutecký</author>
    <author>Michael Hartmann</author>
    <author>Jörn Manz</author>
    <author>Jiřı́ Pittner</author>
    <author>K. Sundermann</author>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>Chemical physics</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>Three dimensional quantum dynamics</value>
    </subject>
    <collection role="jel" number="Y">Miscellaneous Categories</collection>
    <thesisPublisher>SRH Berlin University of Applied Sciences</thesisPublisher>
    <file>https://opus4.kobv.de/opus4-srh/files/563/Ab_initio_three-dimensional.pdf</file>
  </doc>
</export-example>
