TY - INPR A1 - Kaul, Anja A1 - Böllmann, Andrea A1 - Thema, Martin A1 - Kalb, Larissa A1 - Stöckl, Richard A1 - Huber, Harald A1 - Sterner, Michael A1 - Bellack, Annett T1 - Identification of Robust Thermophilic Methanogenic Archaea and Packing Material for High Liquid Hold-Up at Low Volumetric Gas Flow Rates for Use in Trickle-Bed Reactors for Biological Methanation T2 - SSRN Electronic Journal N2 - he hydrogen gas-to-liquid mass transfer is the limiting factor in biological methanation. In a trickle-bed reactor, mass transfer can be increased by high flow velocities in the liquid phase, by adding a packing material with high liquid hold-up, or by choosing methanogenic archaea with a high methane productivity. This study analyzed various packings and methanogenic strains from a hydrodynamic and microbial perspective. By analyzing twelve pure cultures of thermophilic methanogens for their ability to produce high quality methane and to form biofilms on different packings, strains of Methanothermobacter were found to perform better than thus of the genus Methanothermococcus. Best methane production and adherence was observed on DuraTop®, Bioflow 9, and filter foam. DuraTop® and Bioflow 9 had also a high dynamic liquid hold-up, but the maximum hold-up was determined for expanded clay. The ideal combination for use in the ORBIT-trickle-bed reactor was identified as Methanothermobacter thermoautotrophicus IM5 and DuraTop®. KW - Liquid hold-up maximization KW - Methane production KW - Methanothermobacter KW - Methanothermococcus KW - Optimized packing-organism combination Y1 - 2021 U6 - https://doi.org/10.2139/ssrn.3940878 N1 - final peer reviewed article published under: https://doi.org/10.1016/j.biortech.2021.126524 ER - TY - INPR A1 - Heberl, Michael A1 - Withelm, Christian A1 - Kaul, Anja A1 - Rank, Daniel A1 - Sterner, Michael T1 - Prospective Life Cycle Assessment of Biological Methanation in a Trickle-Bed Pilot Plant and a Potential Scale-Up N2 - In this study, a pilot-scale trickle-bed reactor for biological methanation and various scale-up scenarios for 2023 and 2050 were investigated using LCA. A best- and worst-case scenario for technology development until 2050 was evolved using cross consistency analysis and morphological field, based on which the data for the ecological models were determined.The results show that the plant scale-up has a very positive effect on the ecological consequences of methanation. In the best-case scenario, the values are a factor of 23-780 lower than those of the actual plant today. A hot-spot analysis showed that especially electrolysis operation has a large impact on total emissions. The final Monte-Carlo simulation shows that the technology is likely to achieve a low GWP with a median of 104.0 kg CO2-eq / MWh CH4. Y1 - 2023 U6 - https://doi.org/10.2139/ssrn.4635066 N1 - Der Aufsatz wurde peer-reviewd veröffentlich und ist ebenfalls in diesem Repositorium verzeichnet unter: https://opus4.kobv.de/opus4-oth-regensburg/frontdoor/index/index/docId/7349 PB - SSRN ER -