@article{RomeisKostrovKramarenkoetal., author = {Romeis, Dirk and Kostrov, Sergei A. and Kramarenko, Elena Yu and Stepanov, Gennady V. and Shamonin (Chamonine), Mikhail and Saphiannikova, Marina}, title = {Magnetic-field-induced stress in confined magnetoactive elastomers}, series = {Soft Matter}, volume = {16}, journal = {Soft Matter}, number = {39}, publisher = {Royal Society of Chemistry}, address = {Cambridge}, doi = {10.1039/D0SM01337D}, pages = {9047 -- 9058}, abstract = {We present a theoretical approach for calculating the state of stress induced by a uniform magnetic field in confined magnetoactive elastomers of arbitrary shape. The theory explicitly includes the magnetic field generated by magnetizable spherical inclusions in the sample interior assuming a non-linear magnetization behavior. The initial spatial distribution of particles and its change in an external magnetic field are considered. This is achieved by the introduction of an effective demagnetizing factor where both the sample shape and the material microstructure are taken into account. Theoretical predictions are fitted to the stress data measured using a specifically designed experimental setup. It is shown that the theory enables the quantification of the effect of material microstructure upon introducing a specific microstructural factor and its derivative with respect to the extensional strain in the undeformed state. The experimentally observed differences between isotropic and anisotropic samples, compliant and stiff elastomer matrices are explained.}, language = {en} } @article{SavelevBelyaevaChashinetal., author = {Savelev, Dmitrii V. and Belyaeva, Inna A. and Chashin, Dmitri V. and Fetisov, Leonid Y. and Romeis, Dirk and Kettl, Wolfgang and Kramarenko, Elena Yu and Saphiannikova, Marina and Stepanov, Gennady V. and Shamonin (Chamonine), Mikhail}, title = {Giant extensional strain of magnetoactive elastomeric cylinders in uniform magnetic fields}, series = {Materials}, volume = {13}, journal = {Materials}, number = {15}, publisher = {MDPI}, address = {Basel}, issn = {1996-1944}, doi = {10.3390/ma13153297}, pages = {1 -- 17}, abstract = {Elongations of magnetoactive elastomers (MAEs) under ascending-descending uniform magnetic fields were studied experimentally using a laboratory apparatus specifically designed to measure large extensional strains (up to 20\%) in compliant MAEs. In the literature, such a phenomenon is usually denoted as giant magnetostriction. The synthesized cylindrical MAE samples were based on polydimethylsiloxane matrices filled with micrometer-sized particles of carbonyl iron. The impact of both the macroscopic shape factor of the samples and their magneto-mechanical characteristics were evaluated. For this purpose, the aspect ratio of the MAE cylindrical samples, the concentration of magnetic particles in MAEs and the effective shear modulus were systematically varied. It was shown that the magnetically induced elongation of MAE cylinders in the maximum magnetic field of about 400 kA/m, applied along the cylinder axis, grew with the increasing aspect ratio. The effect of the sample composition is discussed in terms of magnetic filler rearrangements in magnetic fields and the observed experimental tendencies are rationalized by simple theoretical estimates. The obtained results can be used for the design of new smart materials with magnetic-field-controlled deformation properties, e.g., for soft robotics.}, language = {en} } @article{RoghaniRomeisGlavanetal., author = {Roghani, Mehran and Romeis, Dirk and Glavan, Gašper and Belyaeva, Inna A. and Shamonin (Chamonine), Mikhail and Saphiannikova, Marina}, title = {Magnetically induced deformation of isotropic magnetoactive elastomers and its relation to the magnetorheological effect}, series = {Physical Review Applied}, volume = {23}, journal = {Physical Review Applied}, number = {3}, publisher = {American Physical Society (APS)}, issn = {2331-7019}, doi = {10.1103/PhysRevApplied.23.034041}, abstract = {Can isotropic magnetoactive elastomers (MAEs) undergo giant magnetically induced deformations and exhibit huge magnetorheological effects simultaneously? In this experimental and theoretical study, we reveal how the macroscopic deformation of MAEs relates to the process of particle restructuring caused by application of a magnetic field. For this purpose, MAE cylinders with different aspect ratios and particle loadings are studied in uniform magnetic fields. The axial deformations of the cylinders are acquired using an optical camera. A unified mean-field model proposed in previous studies is adapted to describe the transition of initially isotropic cylinders into transversely isotropic ones. This mechanical transition is caused by the rearrangement of particles into dense columnar structures aligned with the field and is believed to result in a huge magnetorheological effect. Our model however predicts less than a threefold increase in elastic moduli when evaluated along the field direction. This prediction is based on a careful examination of the shear moduli of studied MAEs and the columnar structures. A weak magnetorheological effect explains significant axial deformations measured in the field direction. A strong magnetorheological effect would hinder axial deformations due to an increase in the modulus by several orders of magnitude. Not only are the moduli and macroscopic deformations influenced by microstructure evolution, but so is the magnetization of particles, which increases as they rearrange into dense columns. With this study, we show that the unified mean-field model provides quantitative access to hidden material properties such as magnetization and stiffness in MAE samples with different shapes and evolving microstructures. Published by the American Physical Society 2025}, language = {en} }