@article{GlavanBelyaevaDrevenšek‐Oleniketal., author = {Glavan, Gašper and Belyaeva, Inna A. and Drevenšek-Olenik, Irena and Shamonin (Chamonine), Mikhail}, title = {Experimental study of longitudinal, transverse and volume strains of magnetoactive elastomeric cylinders in uniform magnetic fields}, series = {Journal of Magnetism and Magnetic Materials}, volume = {579}, journal = {Journal of Magnetism and Magnetic Materials}, publisher = {Elsevier}, issn = {0304-8853}, doi = {10.1016/j.jmmm.2023.170826}, abstract = {Magnetoactive elastomers (MAEs) are promising materials for realization of magnetic field-controlled soft actuators. Herein, a systematic investigation of magnetic field-induced macroscopic deformations of soft MAE cylinders with a diameter of 15 mm in uniform quasi-static magnetic fields directed parallel to the cylinder's axis is reported. The measurements were based on image processing. Thirty-six MAE samples differing in the weight fraction of the iron filler (70 wt\%, 75 wt\% and 80 wt\%), alignment of filling particles, and the aspect ratio (0.2, 0.4, 0.6, 0.8, 1.0 and 1.2) were fabricated. MAE cylinders exhibited high relative change in height (up to 35\% in the field of 485 kA/m) and lateral contraction. The dependence of the maximum extensional strain on the aspect ratio was obtained and compared with theoretical considerations. A concave dent was formed on the free circular base in magnetic fields. This concavity was characterized experimentally. A significant volumetric strain of the order of magnitude of 10\% was calculated in MAEs for the first time. In consequently repeated magnetization cycles, the remanent extensional strain significantly increased after each cycle. The results are qualitatively discussed in the framework of the modern views on the magnetically induced macroscopic deformations of MAEs. The directions of further research are outlined.}, language = {en} } @article{LovšinBrandlGlavanetal., author = {Lovšin, Matija and Brandl, Dominik and Glavan, Gašper and Belyaeva, Inna A. and Cmok, Luka and Coga, Lucija and Kalin, Mitjan and Shamonin (Chamonine), Mikhail and Drevenšek-Olenik, Irena}, title = {Reconfigurable Surface Micropatterns Based on the Magnetic Field-Induced Shape Memory Effect in Magnetoactive Elastomers}, series = {Polymers}, volume = {13}, journal = {Polymers}, number = {24}, publisher = {MDPI}, doi = {10.3390/polym13244422}, abstract = {A surface relief grating with a period of 30 mu m is embossed onto the surface of magnetoactive elastomer (MAE) samples in the presence of a moderate magnetic field of about 180 mT. The grating, which is represented as a set of parallel stripes with two different amplitude reflectivity coefficients, is detected via diffraction of a laser beam in the reflection configuration. Due to the magnetic-field-induced plasticity effect, the grating persists on the MAE surface for at least 90 h if the magnetic field remains present. When the magnetic field is removed, the diffraction efficiency vanishes in a few minutes. The described effect is much more pronounced in MAE samples with larger content of iron filler (80 wt\%) than in the samples with lower content of iron filler (70 wt\%). A simple theoretical model is proposed to describe the observed dependence of the diffraction efficiency on the applied magnetic field. Possible applications of MAEs as magnetically reconfigurable diffractive optical elements are discussed. It is proposed that the described experimental method can be used as a convenient tool for investigations of the dynamics of magnetically induced plasticity of MAEs on the micrometer scale.}, language = {en} } @article{SavelevGlavanBelanetal., author = {Savelev, Dmitrii V. and Glavan, Gašper and Belan, Viktoria O. and Belyaeva, Inna A. and Fetisov, Leonid Y. and Shamonin (Chamonine), Mikhail}, title = {Resonant Magnetoelectric Effect at Low Frequencies in Layered Polymeric Cantilevers Containing a Magnetoactive Elastomer}, series = {Applied Sciences}, volume = {12}, journal = {Applied Sciences}, number = {4}, publisher = {MPDI}, doi = {10.3390/app12042102}, url = {http://nbn-resolving.de/urn:nbn:de:bvb:898-opus4-30637}, pages = {1 -- 13}, abstract = {In this work, the resonance enhancement of magnetoelectric (ME) coupling at the two lowest bending resonance frequencies was investigated in layered cantilever structures comprising a magnetoactive elastomer (MAE) slab and a commercially available piezoelectric polymer multilayer. A cantilever was fixed at one end in the horizontal plane and the magnetic field was applied horizontally. Five composite structures, each containing an MAE layer of different thicknesses from 0.85 to 4 mm, were fabricated. The fundamental bending resonance frequency in the absence of a magnetic field varied between roughly 23 and 55 Hz. It decreased with the increasing thickness of the MAE layer, which was explained by a simple theory. The largest ME voltage coefficient of about 7.85 V/A was measured in a sample where the thickness of the MAE layer was ≈2 mm. A significant increase in the bending resonance frequencies in the applied DC magnetic field of 240 kA/m up to 200\% was observed. The results were compared with alternative designs for layered multiferroic structures. Directions for future research were also discussed.}, language = {en} } @article{GlavanBelyaevaRuwischetal., author = {Glavan, Gašper and Belyaeva, Inna A. and Ruwisch, Kevin and Wollschlaeger, Joachim and Shamonin (Chamonine), Mikhail}, title = {Magnetoelectric Response of Laminated Cantilevers Comprising a Magnetoactive Elastomer and a Piezoelectric Polymer, in Pulsed Uniform Magnetic Fields}, series = {Sensors}, volume = {21}, journal = {Sensors}, number = {19}, publisher = {MDPI}, address = {Basel}, doi = {10.3390/s21196390}, pages = {1 -- 19}, abstract = {The voltage response to pulsed uniform magnetic fields and the accompanying bending deformations of laminated cantilever structures are investigated experimentally in detail. The structures comprise a magnetoactive elastomer (MAE) slab and a commercially available piezoelectric polymer multilayer. The magnetic field is applied vertically and the laminated structures are customarily fixed in the horizontal plane or, alternatively, slightly tilted upwards or downwards. Six different MAE compositions incorporating three concentrations of carbonyl iron particles (70 wt\%, 75 wt\% and 80 wt\%) and two elastomer matrices of different stiffness are used. The dependences of the generated voltage and the cantilever's deflection on the composition of the MAE layer and its thickness are obtained. The appearance of the voltage between the electrodes of a piezoelectric material upon application of a magnetic field is considered as a manifestation of the direct magnetoelectric (ME) effect in a composite laminated structure. The ME voltage response increases with the increasing total quantity of the soft-magnetic filler in the MAE layer. The relationship between the generated voltage and the cantilever's deflection is established. The highest observed peak voltage around 5.5 V is about 8.5-fold higher than previously reported values. The quasi-static ME voltage coefficient for this type of ME heterostructures is about 50 V/A in the magnetic field of approximate to 100 kA/m, obtained for the first time. The results could be useful for the development of magnetic field sensors and energy harvesting devices relying on these novel polymer composites.}, language = {en} } @article{SavelevBelyaevaChashinetal., author = {Savelev, Dmitrii V. and Belyaeva, Inna A. and Chashin, Dmitri V. and Fetisov, Leonid Y. and Romeis, Dirk and Kettl, Wolfgang and Kramarenko, Elena Yu and Saphiannikova, Marina and Stepanov, Gennady V. and Shamonin (Chamonine), Mikhail}, title = {Giant extensional strain of magnetoactive elastomeric cylinders in uniform magnetic fields}, series = {Materials}, volume = {13}, journal = {Materials}, number = {15}, publisher = {MDPI}, address = {Basel}, issn = {1996-1944}, doi = {10.3390/ma13153297}, pages = {1 -- 17}, abstract = {Elongations of magnetoactive elastomers (MAEs) under ascending-descending uniform magnetic fields were studied experimentally using a laboratory apparatus specifically designed to measure large extensional strains (up to 20\%) in compliant MAEs. In the literature, such a phenomenon is usually denoted as giant magnetostriction. The synthesized cylindrical MAE samples were based on polydimethylsiloxane matrices filled with micrometer-sized particles of carbonyl iron. The impact of both the macroscopic shape factor of the samples and their magneto-mechanical characteristics were evaluated. For this purpose, the aspect ratio of the MAE cylindrical samples, the concentration of magnetic particles in MAEs and the effective shear modulus were systematically varied. It was shown that the magnetically induced elongation of MAE cylinders in the maximum magnetic field of about 400 kA/m, applied along the cylinder axis, grew with the increasing aspect ratio. The effect of the sample composition is discussed in terms of magnetic filler rearrangements in magnetic fields and the observed experimental tendencies are rationalized by simple theoretical estimates. The obtained results can be used for the design of new smart materials with magnetic-field-controlled deformation properties, e.g., for soft robotics.}, language = {en} } @article{SavelevBelyaevaChashinetal., author = {Savelev, Dmitrii V. and Belyaeva, Inna A. and Chashin, Dmitri V. and Fetisov, Leonid Y. and Shamonin (Chamonine), Mikhail}, title = {Large Wiedemann effect in a magnetoactive elastomer}, series = {Journal of Magnetism and Magnetic Materials}, volume = {511}, journal = {Journal of Magnetism and Magnetic Materials}, number = {October}, publisher = {Elsevier}, doi = {10.1016/j.jmmm.2020.166969}, abstract = {Large twists of a soft tube (hollow cylinder) in helical magnetic fields are presented for the first time. Such a phenomenon is usually denoted as the Wiedemann effect. The tube is fabricated from a soft magnetoactive elastomer material with the shear modulus of about 56 kPa. The composite material comprises 80 mass\% of micrometer-sized iron particles embedded into a polydimethylsiloxane matrix. The circular magnetic field is generated by an electric current in a straight wire passing through the inner hole of the tube. The maximum value of approximately 350″/cm is observed in a longitudinal magnetic field of a few kA/m overlapped with a circumferential magnetic field of about 1.4 kA/m on the surface of the inner hole. A pronounced hysteresis in the dependence of the Wiedemann effect on the circular magnetic field is found. The ways to enhance the Wiedemann twist in magnetoactive elastomers are discussed. The observed large effect is promising for application in magnetic-field controlled torsional actuators, in particular for soft robotics.}, language = {en} } @misc{PershinaSavelevGlavanetal., author = {Pershina, K. V. and Savelev, Dmitrii V. and Glavan, Gašper and Chashin, Dmitri V. and Belyaeva, Inna A. and Fetisov, Leonid Y. and Shamonin (Chamonine), Mikhail}, title = {The voltage response of a structure comprising a magnetoactive-elastomer cylinder and a piezoelectric material to magnetic field step excitations}, series = {The 4th International Baltic Conference on Magnetism (IBCM 2021) : Svetlogorsk, Russia August 29 - September 2, 2021 : Book of Abstracts}, journal = {The 4th International Baltic Conference on Magnetism (IBCM 2021) : Svetlogorsk, Russia August 29 - September 2, 2021 : Book of Abstracts}, publisher = {Immanuel Kant Baltic Federal University, Kaliningrad, Russia}, pages = {182}, language = {en} } @article{RoghaniRomeisGlavanetal., author = {Roghani, Mehran and Romeis, Dirk and Glavan, Gašper and Belyaeva, Inna A. and Shamonin (Chamonine), Mikhail and Saphiannikova, Marina}, title = {Magnetically induced deformation of isotropic magnetoactive elastomers and its relation to the magnetorheological effect}, series = {Physical Review Applied}, volume = {23}, journal = {Physical Review Applied}, number = {3}, publisher = {American Physical Society (APS)}, issn = {2331-7019}, doi = {10.1103/PhysRevApplied.23.034041}, abstract = {Can isotropic magnetoactive elastomers (MAEs) undergo giant magnetically induced deformations and exhibit huge magnetorheological effects simultaneously? In this experimental and theoretical study, we reveal how the macroscopic deformation of MAEs relates to the process of particle restructuring caused by application of a magnetic field. For this purpose, MAE cylinders with different aspect ratios and particle loadings are studied in uniform magnetic fields. The axial deformations of the cylinders are acquired using an optical camera. A unified mean-field model proposed in previous studies is adapted to describe the transition of initially isotropic cylinders into transversely isotropic ones. This mechanical transition is caused by the rearrangement of particles into dense columnar structures aligned with the field and is believed to result in a huge magnetorheological effect. Our model however predicts less than a threefold increase in elastic moduli when evaluated along the field direction. This prediction is based on a careful examination of the shear moduli of studied MAEs and the columnar structures. A weak magnetorheological effect explains significant axial deformations measured in the field direction. A strong magnetorheological effect would hinder axial deformations due to an increase in the modulus by several orders of magnitude. Not only are the moduli and macroscopic deformations influenced by microstructure evolution, but so is the magnetization of particles, which increases as they rearrange into dense columns. With this study, we show that the unified mean-field model provides quantitative access to hidden material properties such as magnetization and stiffness in MAE samples with different shapes and evolving microstructures. Published by the American Physical Society 2025}, language = {en} } @misc{GlavanBelyaevaShamoninChamonine, author = {Glavan, Gašper and Belyaeva, Inna A. and Shamonin (Chamonine), Mikhail}, title = {On the Piezomagnetism of Magnetoactive Elastomeric Cylinders in Uniform Magnetic Fields: Height Modulation in the Vicinity of an Operating Point by Time-Harmonic Fields [Data set]}, doi = {10.5281/zenodo.13834054}, language = {en} } @misc{GlavanBelyaevaShamoninChamonine, author = {Glavan, Gašper and Belyaeva, Inna A. and Shamonin (Chamonine), Mikhail}, title = {Multiferroic Cantilevers Containing a Magnetoactive Elastomer: Magnetoelectric Response to Low-Frequency Magnetic Fields of Triangular and Sinusoidal Waveform [Data set]}, doi = {10.5281/zenodo.14651784}, language = {en} } @article{GlavanBelyaevaShamoninChamonine, author = {Glavan, Gašper and Belyaeva, Inna A. and Shamonin (Chamonine), Mikhail}, title = {Multiferroic Cantilevers Containing a Magnetoactive Elastomer: Magnetoelectric Response to Low-Frequency Magnetic Fields of Triangular and Sinusoidal Waveform}, series = {Sensors}, volume = {22}, journal = {Sensors}, number = {10}, publisher = {MDPI}, address = {Basel}, doi = {10.3390/s22103791}, pages = {1 -- 17}, abstract = {In this work, multiferroic cantilevers comprise a layer of a magnetoactive elastomer (MAE) and a commercially available piezoelectric polymer-based vibration sensor. The structures are fixed at one end in the horizontal plane and the magnetic field is applied vertically. First, the magnetoelectric (ME) response to uniform, triangle-wave magnetic fields with five different slew rates is investigated experimentally. Time and field dependences of the generated voltage, electric charge, and observed mechanical deflection are obtained and compared for four different thicknesses of the MAE layer. The ME responses to triangular and sinusoidal wave excitations are examined in contrast. Second, the ME response at low frequencies (≤3 Hz) is studied by the standard method of harmonic magnetic field modulation. The highest ME coupling coefficient is observed in the bias magnetic field strength of ≈73 kA/m and it is estimated to be about 3.3 ns/m (ME voltage coefficient ≈ 25 V/A) at theoretically vanishing modulation frequency (f→0 Hz). Presented results demonstrate that the investigated heterostructures are promising for applications as magnetic-field sensors and energy harvesting devices.}, language = {en} } @misc{GlavanBelyaevaShamoninChamonineetal., author = {Glavan, Gašper and Belyaeva, Inna A. and Shamonin (Chamonine), Mikhail and Ruwisch, Kevin and Wollschl{\"a}ger, Joachim}, title = {Magnetoelectric Response of Laminated Cantilevers Comprising a Magnetoactive Elastomer and a Piezoelectric Polymer, in Pulsed Uniform Magnetic Fields [Data set]}, doi = {10.5281/zenodo.14652152}, language = {en} } @misc{GlavanBelyaevaShamoninChamonine, author = {Glavan, Gašper and Belyaeva, Inna A. and Shamonin (Chamonine), Mikhail}, title = {Transient Response of Macroscopic Deformation of Magnetoactive Elastomeric Cylinders in Uniform Magnetic Fields [Data set]}, doi = {10.5281/zenodo.10679499}, language = {en} } @article{GlavanBelyaevaShamoninChamonine, author = {Glavan, Gašper and Belyaeva, Inna A. and Shamonin (Chamonine), Mikhail}, title = {Transient Response of Macroscopic Deformation of Magnetoactive Elastomeric Cylinders in Uniform Magnetic Fields}, series = {Polymers}, volume = {16}, journal = {Polymers}, number = {5, Special Issue Magnetic Polymer Composites: Design and Application II}, publisher = {MDPI}, address = {Basel, Schweiz}, issn = {2073-4360}, doi = {10.3390/polym16050586}, url = {http://nbn-resolving.de/urn:nbn:de:bvb:898-opus4-71067}, pages = {17}, abstract = {Significant deformations of bodies made from compliant magnetoactive elastomers (MAE) in magnetic fields make these materials promising for applications in magnetically controlled actuators for soft robotics. Reported experimental research in this context was devoted to the behaviour in the quasi-static magnetic field, but the transient dynamics are of great practical importance. This paper presents an experimental study of the transient response of apparent longitudinal and transverse strains of a family of isotropic and anisotropic MAE cylinders with six different aspect ratios in time-varying uniform magnetic fields. The time dependence of the magnetic field has a trapezoidal form, where the rate of both legs is varied between 52 and 757 kA/(s·m) and the maximum magnetic field takes three values between 153 and 505 kA/m. It is proposed to introduce four characteristic times: two for the delay of the transient response during increasing and decreasing magnetic field, as well as two for rise and fall times. To facilitate the comparison between different magnetic field rates, these characteristic times are further normalized on the rise time of the magnetic field ramp. The dependence of the normalized characteristic times on the aspect ratio, the magnetic field slew rate, maximum magnetic field values, initial internal structure (isotropic versus anisotropic specimens) and weight fraction of the soft-magnetic filler are obtained and discussed in detail. The normalized magnetostrictive hysteresis loop is introduced, and used to explain why the normalized delay times vary with changing experimental parameters.}, language = {en} }