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The science of measuring airborne volcanic ash concentrations supports research in such fields as atmospheric environmental science and the modeling of atmospheric pollution from volcanoes, and is thus very valuable to the aviation industry. These measurements show large scatter directly traceable to turbulent fluctuations responsible for diffusing volcanic dust. Before semistationary components in observations can be compared to each other or to simulation results, they must be separated from fluctuations. In the design of the separation process, however, neither seasonal or diurnal periodicity nor random disturbance with known properties exists to serve as a guideline. It has been suggested that fluctuations could be eliminated through repeated convolutions of a simple 3-point filter enough times. The number of convolutions is chosen from the change in the rate of increase of a special variability parameter. When semistationary concentrations are separated from fluctuations, their statistics are compared to turbulence parameters and the autocorrelation of the series. The method is demonstrated using three measurement series from Sakurajima, Japan measured in 2013. It is concluded that this new method is simple and trustworthy where knowledge and experience of the environmental parameters can be utilized to support the results. They indicate a variability of 40% in the relative fluctuations of the PM10 and around 20% of the PM2.5. The relative fluctuations may be considered completely random, but normally distributed rather than a white noise with an evenly distributed variance spectrum.
Volcanic ash concentrations in the plume from Sakurajima volcano in Japan are observed from airplanes equipped with optical particle counters and GPS tracking devices. The volcano emits several puffs a day. The puffs are also recorded by the Sakurajima Volcanological Observatory. High concentrations are observed in the puffs and fallout driven by vertical air current, called streak fallout. Puffs dispersion is analyzed by the classical diffusion-advection method and a new gravitational dispersion method. The fluid mechanic of the gravitational dispersion, streak fallout, and classical diffusion-advection theory is described in three separate appendices together with methods to find the time gravitational dispersion constant and the diffusion coefficient from satellite photos. The diffusion-advection equation may be used to scale volcanic eruptions so the same eruption plumes can be scaled to constant flux and wind conditions or two eruptions can be scaled to each other. The dispersion analyses show that dispersion of volcanic plumes does not follow either theories completely. It is most likely diffusion in the interface of the plume and the ambient air, together with gravitational flattening of the plumes core. This means larger boundary concentration gradients and smaller diffusion coefficients than state of the art methods can predict.
Volcanoes emit particles (silicates and sulphate aerosol) and gases (e.g., water and sulphur dioxide) which influence the radiative balance of the atmosphere. The rate at which sulphur dioxide oxidises to sulphate aerosol is poorly constrained and measurements of downwind abundance are required to quantify the rate at which this process occurs.
During July and November 2011, a series of measurements were performed in emissions from Etna Volcano, Sicily, using the University of Applied Sciences (Dusseldorf) research aircraft. Both in situ and remote sensing instrumentation was simultaneously deployed to quantify the down-wind characteristics of gases and particles in the plume emitted by the volcano. In situ particle characteristics were measured using a Grimm 1.109 optical particle counter (microparticles 0.25-32 microns) and Grimm 1320 diffusion electrometer (nanoparticles 25-300 nanometers). Column abundance of sulphur dioxide was measured using a vertically-pointing differential optical absorption spectrometer (DOAS). These measurements were compared to horizontal pathlength-integrated measurements of sulphur dioxide from the Airborne Volcanic Imaging Object Detector (AVOID).
Down-wind plume dispersion was discriminated through a series of aircraft transects below and through the volcanic plume. The emissions contained large amounts of nanoparticles relative to microparticles, which reflects gas-phase nucleation of sulphate aerosol. The AVOID system discriminated horizontal layering of volcanic aerosol at altitudes of up to 12,000 ft from a detection range of >50 km. Plume boundaries were discriminated using a combination of the in situ and DOAS measurements in order to compare to the pathlength-integrated measurements from AVOID.
Aircraft measurements compared with ceilometer measurements during a sahara dust period in Germany
(2015)
A significant Sahara dust event took place at the beginning of April 2014 over large areas of Germany and Europe. The German Weather Service (DWD) detected and monitored the expansion and propagation of this dust cloud with a ceilometer network of more than 50 ceilometers. Moreover, these ceilometers were also able to track the altitude of the dust cloud at the positions of the ceilometers.
Additionally, aircraft measurements over Germany and France were performed with two aircraft by the Duesseldorf University of Applied Sciences. These aircraft were equipped with optical particle counters (OPC) and were able to measure the particle size distribution within the Sahara dust cloud and as a result of this to calculate the particle mass concentration of the dust. The ceilometer measurements and the aircraft measurements complemented each other: whereas the ceilometers gave continuous information about the Sahara dust cloud at the ceilometer positions, the aircraft measurements delivered interpolating results between the ceilometer positions.
Moreover, at several ceilometer positions intercomparison flights were performed by spiraling with the aircraft up or down around the ceilometer laser beam. This gave the unique possibility for comparing the remote sensing results of the ceilometers with the in-situ measurements of the aircraft.
This study shows that a significant high amount of Saharan dust particles was transported over Germany during a several days long episode. Furthermore, the intercomparison study between the German ceilometer network and aircraft measurements results shows a good agreement. A combination of these techniques could help to detect the vertical and horizontal distribution of the dust cloud and additionally the particle mass concentration.
The eruption of the volcano Eyjafjallajökull (Iceland) in 2010 has caused a transportation of an ash dust plume over large areas of Europe. In April 2010 many airports in Europe were closed for several days because of the volcano ash plume and even in May 2010 several German and European airports were closed for shorter periods because of the danger caused by the volcanic ash dust. The VAAC (Volcanic Ash Advisory Center), London, has continuously published graphics of the predicted spread and dispersion of the volcanic ash plume, which were partly basis for the air traffic restrictions in Germany.
In this situation the Laboratory for Environmental Measurement Techniques of the University of Applied Sciences in Duesseldorf has performed 14 measurement flights starting from April 23 2010 to May 21 2010 to get real airborne in-situ dust measurement data over the north-western part of Germany and for comparison with the predicted ash dispersion model data of the VAAC of London in Germany. Moreover, airborne passive DOAS remote sensing measurements have been performed by a mini-DOAS system for SO2-measurements within the plume.
In this paper the results of the airborne optical ash particle measurements as well as the remote sensing SO2 measurements will be reported for situations with and without the volcanic plume over northern Germany in detail. Moreover, the measured dust data will be compared with the model dispersion predictions for the ash plume by the VAAC and with European limit concentrations.
Main conclusions are:
The „ash plume“, found by the aircraft measurement of the Duesseldorf University of Applied Sciences over north western Germany in the “red zone” predicted by the VAAC turned out to be inhomogeneous during the measurement flights
Clusters of ash plume sometimes had only a height extension of several hundred meters or less
Ash substructures with a horizontal extension of ten kilometres up to several tenth of kilometres could be found Vertical double structures of ash plume could be measured by spiral flights and could be observed visually in horizontal direction
Ash plume could be observed visually as small brown layer in horizontal direction
Particles collected during flight could be identified as ash particles by electron microscope analysis and chemical analysis