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Catalytic CO2 methanation: Providing optimal test conditions for kinetic investigations

  • In the context of using renewable energies and recycling climate-changing gases, methanation of CO2 provides one possibility. However, volatile availability of renewable energies for hydrogen production and fluctuating CO2streams from different sources lead to enhanced demand in investigating the influence of dynamic process operation on the catalyst performance, including detailed kinetic characterization. Reliable kinetic measurements require isothermal temperature control and absence of macrokinetic diffusion limitations. Both were investigated in this work while the determination of steady-state kinetic parameters is part of ongoing studies. Furthermore, a detailed analysis with respect to the long-term-stability of the nickel-based catalyst was performed

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Metadaten
Author:Luisa FailingORCiD, Stefan KaluzaORCiD, Peter StrucksORCiD
open access (DINI-Set):open_access
Qualitätssicherung:peer reviewed
open access :Hybrid - Subskriptionszeitschrift
agreement:DEAL Wiley
Fachbereich/Einrichtung:Hochschule Düsseldorf / Fachbereich - Maschinenbau und Verfahrenstechnik
Document Type:Article
Year of Completion:2023
Language of Publication:English
Publisher:Wiley
Parent Title (English):Chemie Ingenieur Technik
Volume:95
Issue:5
First Page:749
Last Page:753
URN:urn:nbn:de:hbz:due62-opus-40026
DOI:https://doi.org/10.1002/cite.202200201
ISSN:1522-2640
Tag:CO2 methanation; Kinetics; Long-term stability; Ni catalyst; Power-to-Gas
Corresponding Author:Stefan Kaluza
Dewey Decimal Classification:6 Technik, Medizin, angewandte Wissenschaften / 62 Ingenieurwissenschaften / 620 Ingenieurwissenschaften und zugeordnete Tätigkeiten
Licence (German):Creative Commons - CC BY - Namensnennung 4.0 International
Release Date:2023/04/26
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