Refine
Keywords
- Gold (2)
- Iridium (2)
- X-ray (2)
- iridium (2)
- mirror (2)
- Biosensor (1)
- Dünne Schicht (1)
- Dünnschichttechnik (1)
- Electrostatics (1)
- Elektret (1)
Document Type
- Conference Proceeding (6) (remove)
Language
- English (6)
Has Fulltext
- no (6)
The need for manipulating matter at its smallest scale has been a hot topic in research for the last decades. As the final goal of arranging single atoms has been achieved, research focuses on two targets: firstly, improving the capabilities of existing technologies towards nanometer resolution and secondly, finding new methods for producing nanostructures in a fast and easy way. Here, we present a new maskless method for sub-micro-patterning of poly(methyl methacrylate) (PMMA) thin films. By applying atomic-force-microscope (AFM) assisted nano-xerography, electric charges were locally injected with an AFM-tip into PMMA. The resulting electrostatic patterns attracted charged gold-nanoparticles, which were selectively deposited onto the PMMA layers with lateral dimensions below 200 nm. In a second step, heat treatment at 275 °C initiated a selective decomposition of the PMMA layer, only observed in PMMA-areas covered with nanoparticles, whereas uncovered areas were not modified by the heat treatment. Analyzing the grooves with the AFM, we found that lines with a width in the sub-micrometer range to several micrometers have successfully been realized. We propose this new and promising method to manufacture nano-grooves used as masking for lift-off processes, for functionalization of underlying areas, or for micro-contact-printing.
Due to the increasing number of diabetes patients worldwide there is an enormous need for accurate, fast and someday also continuous or even closed loop monitoring of blood glucose level. More than 50 years after Clark and Lyons proposed the first glucose enzyme electrodes this concept is still widely in use today. Most concepts use the enzyme glucose oxidase (GOx) that reacts with glucose. These reactions cause a current that is proportional to the amount of glucose present at the sensor. Thus, if the sample volume is known, the blood sugar level can be measured. Although these electrodes have been in use for so long they have the disadvantage of a limited shelf time. In this work we present an enzyme free approach for glucose detection applying ultrathin gold films. According to the basic Fuchs-Sondheimer-theory and other more sophisticated models the resistivity of ultrathin metal films is dominated by scattering effects at their surface. Chemical reactions at the metallic surface are expected to change the conductivity properties and thus these changes can be used to detect molecules. This can be done by creating a self-assembled monolayer at the gold surface. When molecules such as glucose bind to the end groups of this layer the electron scattering and thus the conductivity of the film is expected to change. Ultrathin gold films with a thickness of 6 nm show the largest relative change in resistivity and are thus the preferred film thickness for this application. These gold films show a significant change in resistance when model molecules sodium sulfide and dextran are present, whereas the resistance of a platinum reference electrode does not change significantly.
Future space-based X-ray observatories need to be very lightweight for launcher mass constraints. Therefore they will
use a reduced mirror thickness, which results in the additional requirement of low coating stress to avoid deformation of
the initial precisely shaped mirror substrates. Due to their excellent reflection properties iridium coatings are sometimes
applied for grazing incidence mirrors in astronomical X-ray telescopes. At Aschaffenburg University of Applied
Sciences the coating of thin iridium films by an RF-magnetron sputtering technique is under development. The work is
embedded in collaborations with the Max-Planck-Institute for Extraterrestrial Physics in Germany, the Czech Technical
University in Prague, the Osservatorio Astronomico di Brera in Italy, the German Leibniz Institute for Solid State and
Materials Research in Dresden, and the French Institute Fresnel. Sputtering with different parameters leads to iridium
films with different properties. The current work is focused on the microstructure of the iridium coatings to study the
influence of the substrate and of the argon gas pressure on the thin film growing process. Correlations between coating
density, surface micro-roughness, the crystalline structure of the iridium layers, and the expected reflectivity of the X-ray
mirror as well as coating stress effects are presented and discussed. The final goal of the project is to integrate the
produced prototype mirrors into an X-ray telescope module. On a longer timescale measurements of the mirror modules
optical performance are planned at the X-ray test facility PANTER.
X-ray astronomy uses space-based telescopes to overcome the disturbing absorption of the Earth´s atmosphere. The telescope mirrors are operating at grazing incidence angles and are coated with thin metal films of high-Z materials to get sufficient reflectivity for the high-energy radiation to be observed. In addition the optical payload needs to be light-weighted for launcher mass constrains. Within the project JEUMICO, an acronym for “Joint European Mirror Competence”, the Aschaffenburg University of Applied Sciences and the Czech Technical University in Prague started a collaboration to develop mirrors for X-ray telescopes. The X-ray telescopes currently developed within this Bavarian- Czech project are of Lobster eye type optical design. Corresponding mirror segments use substrates of flat silicon wafers which are coated with thin iridium films, as this material is promising high reflectivity in the X-ray range of interest. The deposition of the iridium films is based on a magnetron sputtering process. Sputtering with different parameters, especially by variation of the argon gas pressure, leads to iridium films with different properties. In addition to investigations of the uncoated mirror substrates the achieved surface roughness has been studied. Occasional delamination of the iridium films due to high stress levels is prevented by chromium sublayers. Thereby the sputtering parameters are optimized in the context of the expected reflectivity of the coated X-ray mirrors. In near future measurements of the assembled mirror modules optical performances are planned at an X-ray test facility.