@article{XuShimizuGuterdingetal.2023, author = {Xu, Han-Xiang and Shimizu, Makoto and Guterding, Daniel and Otsuki, Junya and Jeschke, Harald O.}, title = {Pressure evolution of electronic structure and magnetism in the layered van der Waals ferromagnet CrGeTe3}, series = {Physical Review B}, journal = {Physical Review B}, number = {Vol. 108}, publisher = {American Physical Society}, doi = {https://doi.org/10.1103/PhysRevB.108.125142}, pages = {15}, year = {2023}, abstract = {Layered van der Waals ferromagnets, which preserve their magnetic properties down to exfoliated monolayers, are fueling an abundance of fundamental research and nanoscale device demonstration. CrGeTe3 is a prime example of this class of materials. Its temperature-pressure phase diagram features an insulator-to-metal transition and a significant increase in ferromagnetic Curie-Weiss temperatures upon entering the metallic state. We use density functional theory to understand the magnetic exchange interactions in CrGeTe3 at ambient and elevated pressures. We calculate Heisenberg exchange couplings, which provide the correct ferromagnetic ground state and explain the experimentally observed pressure dependence of magnetism in CrGeTe3. Furthermore, we combine density functional theory with dynamical mean-field theory to investigate the effects of electronic correlations and the nature of the high-pressure metallic state in CrGeTe3.}, language = {en} } @article{ScharfGuterdingHenetal.2025, author = {Scharf, Gili and Guterding, Daniel and Hen, Bar and Sarte, Paul M. and Ortiz, Brenden R. and Rozenberg, Gregory Kh. and Holder, Tobias and Wilson, Stephen D. and Jeschke, Harald O. and Ron, Alon}, title = {Pressure tuning of intrinsic and extrinsic sources to the anomalous Hall effect in CrGeTe3}, series = {Physical Review Research}, volume = {7}, journal = {Physical Review Research}, number = {1}, publisher = {American Physical Society}, doi = {10.1103/PhysRevResearch.7.013127}, pages = {1 -- 8}, year = {2025}, abstract = {The integrated Berry curvature is a geometric property that has dramatic implications for material properties. This study investigates the integrated Berry curvature and other contributions to the anomalous Hall effect in CrGeTe3 as a function of pressure. The anomalous Hall effect is absent in the insulating phase of CrGeTe3 and evolves with pressure in a domelike fashion as pressure is applied. The dome's edges are characterized by Fermi surface deformations, manifested as mixed electron and hole transport. We corroborate the presence of bipolar transport using ab initio calculations, which also predict a nonmonotonic behavior of the Berry curvature as a function of pressure. Quantitative discrepancies between our calculations and experimental results indicate that additional scattering mechanisms, which are also strongly tuned by pressure, contribute to the anomalous Hall effect in CrGeTe3.}, language = {en} }