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This lecture shows an overview of cross-cutting topics whithin the dynamic sector of hydrogen technologies including European and other international strategies, legal and policy frameworks, networks and relevant stakeholders, research and demo-projects, regulations, codes & Standards as well as initiatives and associations concerning hydrogen safety and education.
Im hier vorliegenden Bericht wurde im Rahmen einer umfassenden Literaturrecherche der nationale und internationale Stand von Wissenschaft und Technik hinsichtlich Behälterkonzepten und Behälteranforderungen erfasst. Dabei wurde eine umfangreiche Dokumentensammlung zusammengestellt und sortiert, die als Quellenbasis für alle weiteren Arbeiten zur Verfügung steht. Die Auswertung der gesammelten Informationen resultiert in einem Überblick über internationale Behälterentwicklungen sowie einer detaillierten Übersicht über die Behälterkonzepte und die ihnen zugrundeliegenden Anforderungskataloge aus elf fortgeschrittenen Endlagerprogrammen.
Der Bericht zum Arbeitspaket 3 baut auf den Ergebnissen der internationalen Recherche (AP1) sowie der Zusammenstellung der Randbedingungen und Beanspruchungsgrößen für die Endlagerbehälter (AP2) auf. Die Anforderungen an die Behälter – regulatorische, betriebliche sowie solche aus der Standortgeologie und den Einwirkungen und Prozessen, denen die Behälter ausgesetzt sind – werden hergeleitet und systematisch dargestellt.
Die für das Endlagersystem zu betrachtenden Nutzungsphasen werden aus den regulatorischen Anforderungen hergeleitet und charakterisiert. Die Einwirkungen auf die Behälter in den drei potenziellen Wirtsgesteinen sowie die sich für die Erfüllung der Sicherheitsfunktionen des Behälters als Teil des Endlagersystems ergebenden Behälterfunktionen werden ebenfalls wirtsgesteins- und zeitphasenabhängig betrachtet. Schließlich werden aus den Einwirkungen auf die Behälter und den Anforderungen an die Behälterfunktionen auch quantifizierbare Behälterfunktionen für alle drei potenziellen Wirtsgesteine abgeleitet.
The German nuclear waste management strategy consists of dry interim storage of spent fuel inside dual purpose casks and its subsequent direct final disposal in a deep geological repository. Interim storage is limited to 40 years so far, but will have to be extended until repository site selection and operation is concluded, potentially up to 100 years. In this context, research on the long term performance of safety relevant cask components and fuel rod integrity during such extended periods of time is of outmost importance. The barrier function of the fuel cladding depends on its integrity under operational and accidental conditions along with storage and subsequent transportation and is mainly affected over time by altering of the cladding microstructure and by thermo-mechanical conditions during reactor operation and subsequent wet and dry storage.
This paper focuses on failure mechanisms regarding cladding embrittlement caused by physical phenomena concerning hydrogen dissolution and precipitation of hydrides in the zirconium matrix. Within this context, potential cladding integrity issues under extended interim storage conditions followed by transportation are emphasized.
Delayed hydride cracking (DHC) is a well-known time-dependent temperature-activated phenomenon failure mechanism of the fuel cladding during reactor operation. The phenomenon consists of hydrogen diffusion and hydride precipitation at the tip of an initial crack and the propagation of the crack to an approximate distance equal to the length of the hydride. This failure mechanism is temperature-activated phenomenon and enhances along with thermal cycling of the fuel cladding, e. g. during reactor shutdowns. DHC shows limited relevance under quasi static storage conditions with continuously lowering temperatures. However, the literature points that DHC may occur when the temperature during storage decreases to a certain level after some decades and in combination with stress concentrations in the cladding material.
When spent fuel is transferred to dry storage by vacuum drying, the cladding temperature raises up to peak temperatures of ~370°C. Under these conditions, hydrides dissolute into the zirconium matrix up to the solubility limit defined by the peak temperature and this amount of hydrogen can precipitate in a radial re-oriented fashion due to the temperature decrease during storage. Cladding materials with radially precipitated hydrides show significant embrittlement. Radially oriented hydrides are perpendicularly oriented to hoop stresses representing the most critical configuration. Brittle failure of the cladding then occurs by crack propagation through radially oriented hydrides and finally through the zirconium matrix. The susceptibility to radial hydride precipitation depends on cladding material type and microstructure, hydrogen content, pre-drying hydride distribution, irradiation conditions, and temperature and stress histories during drying and storage operations.
This paper addresses major considerations concerning spent fuel cladding embrittlement due to hydride precipitation with regard to the boundary conditions of dry spent fuel storage in Germany. Analytical, numerical, and experimental approaches are to be discussed by BAM in order to identify the specific needs for future R&D work in that area with the purpose to provide the necessary data base for proper safety demonstration and evaluation along with future extended storage licensing procedures.
The presentation explains recent administrative developments in Germany concerning nuclear waste management and adresses national and European R&D funding concepts. National and international collaboration is explained followed by the latest update on long term metal seal investigations at BAM. Finally, fuel cladding failure mechanisms during long term dry storage and related R&D initiatives at BAM are explained.
The German nuclear waste management strategy consists of dry interim storage of spent fuel inside dual purpose casks and its subsequent direct final disposal in a deep geological repository. Interim storage is limited to 40 years so far, but will have to be extended until repository site selection and operation is concluded, potentially up to 100 years. In this context, research on the long term performance of safety relevant cask components and fuel rod integrity during such extended periods of time is of outmost importance. The barrier function of the fuel cladding depends on its integrity under operational and accidental conditions along with storage and subsequent transportation and is mainly affected over time by altering of the cladding microstructure and by thermo-mechanical conditions during reactor operation and subsequent wet and dry storage.
This paper focuses on failure mechanisms regarding cladding embrittlement caused by physical phenomena concerning hydrogen dissolution and precipitation of hydrides in the zirconium matrix. Within this context, potential cladding integrity issues under extended interim storage conditions followed by transportation are emphasized.
Delayed hydride cracking (DHC) is a well-known time-dependent temperature-activated phenomenon failure mechanism of the fuel cladding during reactor operation. The phenomenon consists of hydrogen diffusion and hydride precipitation at the tip of an initial crack and the propagation of the crack to an approximate distance equal to the length of the hydride. This failure mechanism is temperature-activated phenomenon and enhances along with thermal cycling of the fuel cladding, e. g. during reactor shutdowns. DHC shows limited relevance under quasi static storage conditions with continuously lowering temperatures. However, the literature points that DHC may occur when the temperature during storage decreases to a certain level after some decades and in combination with stress concentrations in the cladding material.
When spent fuel is transferred to dry storage by vacuum drying, the cladding temperature raises up to peak temperatures of ~370°C. Under these conditions, hydrides dissolute into the zirconium matrix up to the solubility limit defined by the peak temperature and this amount of hydrogen can precipitate in a radial re-oriented fashion due to the temperature decrease during storage. Cladding materials with radially precipitated hydrides show significant embrittlement. Radially oriented hydrides are perpendicularly oriented to hoop stresses representing the most critical configuration. Brittle failure of the cladding then occurs by crack propagation through radially oriented hydrides and finally through the zirconium matrix. The susceptibility to radial hydride precipitation depends on cladding material type and microstructure, hydrogen content, pre-drying hydride distribution, irradiation conditions, and temperature and stress histories during drying and storage operations.
This paper addresses major considerations concerning spent fuel cladding embrittlement due to hydride precipitation with regard to the boundary conditions of dry spent fuel storage in Germany. Analytical, numerical, and experimental approaches are to be discussed by BAM in order to identify the specific needs for future R&D work in that area with the purpose to provide the necessary data base for proper safety demonstration and evaluation along with future extended storage licensing procedures.
The current German waste management strategy consists of dry interim storage of spent fuel inside dual purpose casks at various sites and its subsequent direct final disposal in a deep geological repository. Interim facilities are licensed for up to 40 years of operation but this storing period will have to be extended until repository site selection and operation is concluded, potentially up to 100 years. In this context, research on long term mechanical behavior of fuel cladding and cask components during extended interim storage and transportation to a final repository are of outmost importance.
Barrier properties of the fuel cladding depend on its integrity which is affected over time by thermo-mechanical loads and by microstructure altering including potential embrittlement caused by re-oriented hydride precipitation. Experimental and numerical investigations have been performed by the international research community in order to predict the degree of cladding embrittlement against storage time. Results have shown that embrittlement of cladding materials is governed by the concentration, orientation and size of precipitated hydrides. Nevertheless, the existing variety of fuel materials and assemblies available on the market and the many parameters effecting hydride precipitation do not allow sufficient reliable safety predictions in the long term without further investigation.
Thus, knowledge on cladding integrity over storage time and during subsequent transportation is to be gained taking into consideration the relevant fuel and cladding material types as well as cladding temperatures along with peak values during cask drying and cooling rates during storage periods. Expected research results will increase the accuracy of cladding safety analysis. This paper summarizes the current German status regarding extended interim storage and how BAM is going to identify and address potential cladding integrity issues in the long term.
The presentation explains the requirements, process and challenges of the container design testing procedures for the Konrad repository, where low and intermediate level radioactive waste is planned to be disposed of beginnung end of 2022. BAM performs container design testing for more than 30 years whether analytically or experimentally. The challenges of the complex Konrad requirements concerning their proper interpretation and application is discussed in this presentation.
Safety of long term containment and storage of radioactive waste is an essential issue, which is increasingly gaining international attention. Extending interim storage beyond initial license periods is one of the major challenges worldwide.
BAM has been involved in all kinds of radioactive waste container safety evaluation for storage and transportation including their long term performance from the very beginning. Today, all work related to the safe management of radioactive waste is linked by the activity field “Nuclear Waste Management” within the Focus Area “Energy” at BAM and in conjunction with a research strategy and agenda. Most recently, the working group “Long Term Safety of Container Systems and Components” was established to launch and perform research projects related to safety issues concerning the extended interim storage of radioactive waste.
For example, within our project LaMEP, we investigate ageing effects of metal and elastomer seals as well as polymeric neutron shielding materials, which are container components that fulfil major safety functions. The results of the experiments help to understand the long term behaviour of these components. Likewise, our project BRUZL started at BAM in 2018 with the aim of developing a fracture mechanics approach to understand and describe a potential brittle failure mechanism of fuel cladding during long-term interim storage. BAM also contributes to the GRS project “Development of methods and models and international exchange for safety evaluation in the frame of interim storage of radioactive waste”. Additionally, BAM is involved in several international research programmes dealing with extended interim storage, such as the European Joint Programme on Radioactive Waste Management (EURAD), the Extended Storage Collaboration Program (ESCP) and IAEA Coordinated Research Projects.
The present contribution provides a comprehensive overview of BAM research activities contributing to national and international gap analyses and to filling knowledge gaps regarding the safe long term management of radioactive waste.
Im Vorhaben "KoBrA" sollen aus bestehenden Anforderungen für endlagerfähige Behälter und aus internationalen Erfahrungen ein aktueller Stand auf dem Gebiet der Behälterforschung für HLW/SF-Behälter ermittelt und generische Vorschläge für einen deutschen HLW/BE-Endlagerbehälter in den drei potentiellen Wirtsgesteinen (Kristallin, Ton oder Salz) erarbeitet werden. Im Arbeitspaket 1 wird dafür eine umfassende Literaturrecherche zu internationalen Behälterkonzepten durchgeführt, deren erste Ergebnisse hier präsentiert werden.