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The excellent mechanical properties of elastomer seals at a wide range of temperatures as well as their high versatility and recovery potential under several load conditions make these materials well suitable for the application in containers designed for transport and disposal of negligible heat generating radioactive waste. While a seal exchange at defined intervals is typical in many conventional applications, it is impossible or at least hard to perform when principles of minimization of radiation exposure have to be considered which prohibit an avoidable cask handling. An extensive knowledge of the change of the elastomer properties during aging and the availability of reliable end-of-lifetime criteria to guarantee the safe enclosure of the radioactive material for the required time are mandatory. As BAM is involved in most of the national cask licensing procedures and in the evaluation of cask-related long-term safety issues, great efforts have already been made and are still ongoing to scientifically support this task.
Among other representative types of elastomers, specimen made from ethylene propylene diene rubber (EPDM) were tested before, during and after aging to capture the with respect to application most important of their complex mechanical properties.
Exemplary results of these investigations were used to calibrate material models implemented in the commercial finite element software ABAQUS/Standard®. The finite element model already presented in previous works uses a sequential temperature displacement coupling. The calculated compression stress relaxation (CSR) and compression set (CS) values do satisfactorily match the experimental results.
In many investigations performed at BAM both values (CSR and CS) were identified as key indicators of elastomer’s long-term performance.
However, the possibility to correlate these equivalent indicators with performance values such as tightness and leakage rate, measurable in the mounted state, is an important goal of our future work. In the presented study the ABAQUS® feature of “pressure penetration” is introduced in the suggested finite element model for this purpose. It provides the possibility to simulate the penetration of a gas into a possible gap between flange and O-ring causing an opening of a leakage path. Three dimensional and axis-symmetric finite element models were generated to represent flat and grooved flanges of different dimensions.
The sensitivity of the feature to several input parameters is investigated and the observed behavior of the O-ring is correlated with the results of performed leakage tests.
Elastomer seals are mounted as barrier seals in lid systems of containers designed for transport and disposal of negligible heat generating radioactive waste and as auxiliary seals in spent fuel storage and transportation casks (dual purpose casks (DPC)). When the behavior of mounted seals under normal and hypothetical accident conditions of disposal and transport is to be simulated, a comprehensive knowledge of their complex mechanical properties at every state of aging is necessary. In previous works, BAM’s efforts in experimental investigations on specimen artificially aged at different temperatures and times and the implementation of the found results in finite element material models were presented. Additionally, our approaches to reproduce the aging process itself and to extrapolate the results of artificially accelerated aging to longer times were presented. Numerical simulations have shown that the behavior of the seal during mounting and one-sided pressurizing and the resulting performance values such as leakage rate strongly depend on the coefficient of friction (COF) between flange and seal. The friction coefficient, in turn, depends on the aging state of the elastomer material as several publications suggest (see below).
Dynamic COF between an exemplary ethylene propylene diene rubber (EPDM) material and a stainless steel ball were determined by using a self-designed linear oscillation tribometer. Unaged and artificially aged EPDM specimen stored for 30 days and 100 days at a temperature of 150 °C were tested. A stainless steel ball (d=10 mm) is brought in contact with the specimen’s surface und loaded by normal forces of 2.5 N, 5 N, 10 N and 20 N. During a reciprocating movement of the EPDM sheet, the horizontal force/friction force is continuously measured, and the COF can be derived.
It is well known that friction is a complex phenomenon especially in soft materials. It cannot be excluded that the measured friction force is influenced by additional force components, resulting from the ball’s grooving through the elastomer’s surface. This force depends on the penetration depth of the ball and on the resistance of the elastomer in its different states of aging. The latter results from microstructural changes i.e., chain scission and additional crosslinking that occur during aging which in turn influence the softening or hardening of the material.
A finite element (FE) ABAQUS® model was developed to reproduce the measurement process. It should help to better understand the physical mechanisms and to quantify the percentage of measured forces resulting from real friction on the one hand and forces resulting from unintended side effects that could falsify the result on the other hand. The behavior of the elastomer in its different states of aging is reproduced by a FE material model already presented in previous works of BAM.
Testing and numerical simulation of elastomeric seals under consideration of time dependent effects
(2016)
Due to delays in the siting procedure to establish a deep geological repository for spent nuclear fuel and high level waste and in construction of the already licensed Konrad repository for low and intermediate level waste, extended periods of interim storage will become more relevant in Germany. BAM is involved in most of the cask licensing procedures and is responsible for the evaluation of cask-related long-term safety issues. Elastomeric seals are widely used as barrier seals for containers for low and intermediate level radioactive waste. In addition they are also used as auxiliary seals in spent fuel storage and transportation casks (dual purpose casks (DPC)).
To address the complex requirements resulting from the described applications, BAM has initiated several test programs for investigating the behavior of elastomeric seals. These include experiments concerning the hyperelastic and viscoelastic behavior at different temperatures and strain rates, the low temperature performance down to -40°C, the influence of gamma irradiation and the aging behavior.
The first part of the paper gives an overview of these tests, their relevant results and their possible impact on BAM’s work as a consultant in the framework of approval and licensing procedures.
The second part presents an approach of the development of a finite element model using the finite element code ABAQUS®. The long-term goal is to simulate the complex elastomeric behavior in a complete lid closure system under specific operation and accident conditions.
The Federal Institute for Materials Research and Testing (BAM) is assessing the mechanical and thermal safety performance of packages for the transport of radioactive materials. Drop testing and numerical calculations are usually part of the safety case concepts, where BAM is performing the regulatory tests at their own test facility site.
Among other mechanical tests the 1 meter drop onto a steel puncture bar shall be considered for accident safe packages. According to the IAEA regulations “the bar shall be of solid mild steel of circular section, 15.0 ± 0.5 cm in diameter and 20 cm long, unless a longer bar would cause greater damage…”.
Particularly with regard to the German transport- and storage cask designs, often made from ductile cast iron, an accurate determination of the puncture bar length to guarantee a load impact covering the worst case scenario can be imperative. If the fracture mechanical proof for the cask material shall be provided by a test, small deviations in the concentrated load applied can be decisive for the question if the cask fails or not.
The most damaging puncture bar length can be estimated by iterative procedure in numerical simulations. On the one hand, a sufficient puncture bar length shall guarantee that shock absorbers or other attachments do not prevent or reduce the local load application to the package, on the other hand, a longer and thus less stiff bar causes a smaller maximum contact force. The contrary influence of increasing puncture bar length and increasing effective drop height shall be taken into account if a shock absorber is directly placed in the target area. The paper presents a numerical approach to identify the bar length that causes maximum damage to the package. Using the example of two typical package masses the sensitivity of contact forces and puncture bar deformations to the initial length are calculated and assessed with regard to the international IAEA package safety requirements.
Due to their high versatility and recovery potential under several load conditions, seals made from elastomers are widely used as barrier seals in containers for low and intermediate level radioactive waste and as auxiliary seals in spent fuel storage and transportation casks (dual purpose casks (DPC)). In DPC, elastomer seals allow leakage rate measurements of metal barrier seals for demonstration of their proper assembly conditions and performance.
For spent fuel and high level waste as well as for low and intermediate level waste, long time periods will be required before final disposal will be available. Therefore, the long-term behavior of elastomer seals can be an important issue when the cask’s suitability for an extended interim storage period has to be assessed.
During the licensed interim storage duration, the requested leakage rate has to be maintained under any static and dynamic load conditions. A sufficient resilience, the capability of seals to compensate a (rapid) partial release was identified as an important end-of-lifetime criterion.
In the framework of extensive aging and testing programs at BAM, specimen made from representative types of elastomer (EPDM, FKM) were aged for several years at different temperatures ranging from 23 °C to 150 °C. One aim of the experiments was to determine an end-of-lifetime criterion correlated to leakage as the point of seal failure. As the seals remained leak-tight under static conditions even after advanced material degradation, a more demanding leakage test set-up was constructed that allowed a rapid partial release of the seal. This device enables a release of the O-ring by approx. 0.2 mm from 25 % to 23 % compression in less than one second during the pressure rise measurement. If the resilience of the seal has decreased past a certain point, the seal cannot follow the decompression fast enough and a leak path can open. Using a finite element (FE) material model derived earlier from different material tests, this process was simulated with a 3D FE model, reproducing the essential characteristics of the test device.
The FE-model enables the analyzation of the occurring global mechanisms if a leak path opens. The capability of the seals to follow the lifted flange and the subsequent run of compression force depending on the current state of aging are illustrated. The findings of the simulation are correlated and discussed with respect to the pressure rise measurements.
Among other mechanical tests the 1 meter drop onto a steel puncture bar shall be considered for accident safe packages for the transport of radioactive material. According with the IAEA regulations “the bar shall be of solid mild steel of circular section, 15.0 ± 0.5 cm in diameter and 20 cm long, unless a longer bar would cause greater damage…”. The most damaging puncture bar length can be estimated by iterative processes in numerical simulations. On the one hand, a sufficient puncture bar length has to guarantee that shock absorbers or other attachments do not prevent or reduce the local load application to the package, on the other hand, a longer and thus less stiff bar causes a smaller maximum contact force. The contrary influence of increasing puncture bar length and increasing effective drop height shall be taken into account if a shock absorber is directly placed in the target area. The paper presents a numerical approach to identify the bar length that causes maximum damage to the package. Using the example of two typical package masses the sensitivity of contact forces and puncture bar deformations to the initial length are calculated and assessed with regard to the international IAEA package safety requirements.