TY - RPRT A1 - Caruso, Stefano A1 - Vlassopoulos, Efstathios A1 - Dagan, Ron A1 - Fiorito, Luca A1 - Herm, Michel A1 - Jansson, Peter A1 - Kromar, Marjan A1 - Király, Márton A1 - Leppanen, Jaakko A1 - Feria Marquez, Francisco A1 - Metz, Volker A1 - Papaioannou, Dimitrios A1 - Herranz, Luis Enrique A1 - Rochman, Dimitri A1 - Schillebeeckx, Peter A1 - Seidl, Marcus A1 - Hernandez Solis, Augusto A1 - Stankovskiy, Alexey A1 - Alvarez Velarde, Francisco A1 - Verwerft, Marc A1 - Rodriguez Villagra, Nieves A1 - Zencker, Uwe A1 - Žerovnik, Gasper T1 - EURAD - Work Package 8 - Deliverable 8.1 - State-of-the-art report N2 - A state-of-the-art (SOTA) review on characterisation of spent nuclear fuel (SNF) properties in terms of source term and inventory assessment (neutron, gamma-ray emission, decay heat, radionuclide inventory, elemental content) and in terms of out-of-core fuel performance (cladding performance and fuel integrity in view of the safety criteria for SNF interim storage, transport and canister packaging) using several numerical and experimental approaches and methodologies is presented. This SOTA report is a result of the spent fuel characterisation (SFC) work package as part of the European Joint Programme on Radioactive Waste Management (EURAD), which offers an overview of the status of knowledge in the field of SNF characterisation and assessment during the pre-disposal phase. The document aims to focus on the current safety-significant gaps and related challenges, providing a direct link to the goals of the mandated actors of EURAD. The report is expected to be used by all EURAD colleagues in their national programmes as a key resource for knowledge management programmes and to contribute to demonstrating and documenting the state-of-the-art. KW - Radioactive waste management KW - Spent fuel characterisation KW - Extended interim storage KW - Predisposal PY - 2022 UR - https://www.ejp-eurad.eu/publications/eurad-d81-state-art-report SP - 1 EP - 112 PB - Agence Nationale pour la Gestion des Déchets Radioactifs (ANDRA) CY - Châtenay-Malabry AN - OPUS4-59154 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - CONF A1 - Liu, Yung A1 - Völzke, Holger A1 - Zencker, Uwe A1 - Jaunich, Matthias T1 - Cooperation in Advanced Technologies Associated with the Back End of Nuclear Fuel Cycle N2 - A Memorandum of Understanding (MOU) between Argonne National Laboratory (Argonne) and the German Bundesanstalt für Materialforschung und -prüfung (BAM) was signed in October 2014. Its objectives are to promote cooperation among scientists and specialists at Argonne and BAM and establish a framework for collaboration in advanced technologies associated with the back end of the nuclear fuel cycle. Collaborative activities involving Argonne and BAM may be implemented through the promotion of joint research activities and scientific workshops and conferences; exchange of technical information; and visits by scientists, specialists, and graduate, postgraduate, and Ph.D. students. The MOU was renewed in January 2020 for another five years. Highlights of the progress and achievements are provided in identified topical areas for collaboration on ageing management guidance, storage, transportation and disposal R&D, joint conference activities, and conclude with the benefits of the MOU in fostering Argonne and BAM collaboration. T2 - 26th International Conference on Structural Mechanics in Reactor Technology - SMiRT 26 CY - Potsdam, Germany DA - 10.07.2022 KW - Nuclear fuel cycle KW - Back end KW - Spent fuel performance KW - Storage KW - Transportation PY - 2022 SP - 1 EP - 10 AN - OPUS4-55861 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - JOUR A1 - Ruiz-Hervias, J. A1 - Simbruner, Kai A1 - Cristobal-Beneyto, M. A1 - Perez-Gallego, D. A1 - Zencker, Uwe T1 - Failure mechanisms in unirradiated ZIRLO® cladding with radial hydrides N2 - The purpose of this paper is to investigate the relationship between hydride morphology, in particular the presence of radial hydrides (RHs), stress state and failure mechanisms associated with the ring compression test (RCT). Samples of ZIRLO®cladding were pre-hydrided and subjected to thermo-mechanical treatments to precipitate long radial hydrides. The results show that the reorientation treatment was very successful. A considerable fraction of RHs was generated, the radial hydride continuity factor being around 80 to 90% of the wall thickness. The samples with reoriented hydrides were tested using the RCT at room temperature. Macroscopic brittle failure was observed with sudden load drops for displacements around 0.5 mm, with a calculated “offset strain”between 0.5 and 1%. Crack nucleation occurs in RHs located in regions with the highest values of hoop stress. These locations are the inner diameter of cladding at the vertical plane of the sample (12 and 6 o’clock positions) and the outer diameter at the horizontal plane (3 and 9 o’clock positions). Noticeable load drops in the RCT are associated with unstable crack propagation events through the radial hydride network, the crack front reaching up to 90% of the wall thickness in some cases. The failure micro-mechanism is quasi-cleavage in the hydrides and micro-void nucleation, growth and coalescence in the Zr matrix, with ductile tearing patches connecting neighboring hydrides. The main conclusion is that radial hydride metrics is not the only parameter that determines cladding failure in the presence of RHs, but the interaction between the location and continuity of RHs and the stress normal to the hydride (the hoop stress in this case). Consequently, if a radial hydride is located at a position within the cladding where the hoop stress is small, a crack will not be initiated easily in the RCT. KW - ZIRLO® KW - Cladding Embrittlement KW - Radial Hydrides KW - Failure Mechanism KW - Ring compression test PY - 2021 DO - https://doi.org/10.1016/j.jnucmat.2020.152668 SN - 0022-3115 VL - 544 SP - 152668 PB - Elsevier B.V. AN - OPUS4-52000 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - CONF A1 - Simbruner, Kai A1 - Billone, M. C. A1 - Zencker, Uwe A1 - Liu, Y. Y. A1 - Völzke, Holger T1 - Brittle Failure Analysis of High-Burnup PWR Fuel Cladding Alloys N2 - The general aim of this research is the development of methods for predicting mechanical behavior and identification of limiting conditions to prevent brittle failure of high-burnup (HBU) pressure water reactor (PWR) fuel cladding alloys. A finite element (FE) model of the ring compression test (RCT) was created to analyze the failure behavior of zirconium-based alloys with radial hydrides during the RCT. An elastic-plastic material model describes the zirconium alloy. The stress-strain curve needed for the elastic-plastic material model was derived by inverse finite element analyses. Cohesive zone modeling is used to reproduce sudden load drops during RCT loading. Based on the failure mechanism in non-irradiated ZIRLO® claddings, a micro-mechanical model was developed that distinguishes between brittle failure along hydrides and ductile failure of the zirconium matrix. Two different cohesive laws representing these types of failure are present in the same cohesive interface. The key differences between these constitutive laws are the cohesive strength, the stress at which damage initiates, and the cohesive energy, which is the damage energy dissipated by the cohesive zone. Statistically generated matrix-hydride distributions were mapped onto the cohesive elements and simulations with focus on the first load drop were performed. Computational results are in good agreement with the RCT results conducted on high-burnup M5® samples. It could be shown that crack initiation and propagation strongly depend on the specific configuration of hydrides and matrix material in the fracture area. T2 - 26th International Conference on Structural Mechanics in Reactor Technology - SMiRT 26 CY - Potsdam, Germany DA - 10.07.2022 KW - Cladding Embrittlement KW - Cohesive Zone Modelling KW - Spent Nuclear Fuel KW - Ring Compression Test PY - 2022 SP - 1 EP - 10 AN - OPUS4-55434 LA - deu AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - JOUR A1 - Simbruner, Kai A1 - Billone, Michael C. A1 - Zencker, Uwe A1 - Liu, Yung Y. A1 - Völzke, Holger T1 - Brittle failure analysis and modeling of high-burnup PWR fuel cladding alloys N2 - The aim of this research is the development of methods for predicting mechanical behavior and identification of limiting conditions to prevent brittle failure of high-burnup (HBU) pressure water reactor (PWR) fuel cladding alloys. A finite element (FE) model of the ring compression test (RCT) was created to analyze the failure behavior of zirconium-based alloys with radial hydrides during the RCT. An elastic-plastic material model describes the zirconium alloy. The stress-strain curve needed for the elastic-plastic material model was derived by inverse finite element analyses. Cohesive zone modeling is used to reproduce sudden load drops during RCT loading. Based on the failure mechanism in non-irradiated ZIRLO® claddings, a micro-mechanical model was developed that distinguishes between brittle failure along hydrides and ductile failure of the zirconium matrix. Two different cohesive laws representing these types of failure are present in the same cohesive interface. The key differences between these constitutive laws are the cohesive strength, the stress at which damage initiates, and the cohesive energy, which is the damage energy dissipated by the cohesive zone. Statistically generated matrix-hydride distributions were mapped onto the cohesive elements and simulations with focus on the first load drop were performed. Computational results are in good agreement with the RCT results conducted on high-burnup M5® samples. It could be shown that crack initiation and propagation strongly depend on the specific configuration of hydrides and matrix material in the fracture area. KW - Cladding KW - Radial hydrides KW - Ring compression test KW - Cohesive zone model PY - 2024 DO - https://doi.org/10.1515/kern-2024-0109 SN - 2195-8580 SP - 1 EP - 9 PB - Walter de Gruyter GmbH AN - OPUS4-62409 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - JOUR A1 - Sjöland, A. A1 - Christensen, P. A1 - Zetterström Evins, L. A1 - Bosbach, D. A1 - Duro, L. A1 - Farnan, I. A1 - Metz, V. A1 - Zencker, Uwe A1 - Ruiz-Hervias, J. A1 - Rodriguez-Villagra, N. A1 - Kiraly, M. A1 - Schillebeeckx, P. A1 - Rochman, D. A1 - Seidl, M. A1 - Dagan, R. A1 - Verwerft, M. A1 - Herranz Puebla, L. E. A1 - Hordynskyi, D. A1 - Feria, F. A1 - Vlassopoulos, E. T1 - Spent nuclear fuel management, characterisation, and dissolution behaviour: progress and achievement from SFC and DisCo N2 - SFC is a work package in Eurad that investigates issues related to the properties of the spent nuclear fuel in the back-end of the nuclear fuel cycle. Decay heat, nuclide inventory, and fuel integrity (mechanical and otherwise), and not least the related uncertainties, are among the primary focal points of SFC. These have very significant importance for the safety and operational aspect of the back-end. One consequence is the operation economy of the back-end, where deeper understanding and quantification allow for significant optimization, meaning that significant parts of the costs can be reduced. In this paper, SFC is described, and examples of results are presented at about half-time of the work package, which will finish in 2024. The DisCo project started in 2017 and finished in November 2021 and was funded under the Horizon 2020 Euratom program. It investigated if the properties of modern fuel types, namely doped fuel, and MOX, cause any significant difference in the dissolution behavior of the fuel matrix compared with standard fuels. Spent nuclear fuel experiments were complemented with studies on model materials as well as the development of models describing the solid state, the dissolution process, and reactive transport in the near field. This research has improved the understanding of processes occurring at the interface between spent nuclear fuel and aqueous solution, such as redox reactions. Overall, the results show that from a long-term fuel matrix dissolution point of view, there is no significant difference between MOX fuel, Cr+Al-doped fuel, and standard fuels. KW - Spent nuclear fuel management KW - Spent fuel characterization KW - Dissolution behaviour PY - 2023 UR - https://nbn-resolving.org/urn:nbn:de:kobv:b43-572461 DO - https://doi.org/10.1051/epjn/2022029 SN - 2491-9292 VL - 9 SP - 1 EP - 12 PB - EDP Sciences CY - Les Ulis Cedex, France AN - OPUS4-57246 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - RPRT A1 - Vlassopoulos, Efstathios A1 - Dagan, Ron A1 - Fiorito, Luca A1 - Herm, Michel A1 - Jansson, Peter A1 - Kromar, Marjan A1 - Király, Márton A1 - Leppanen, Jaakko A1 - Feria Marquez, Francisco A1 - Metz, Volker A1 - Papaioannou, Dimitrios A1 - Herranz, Luis Enrique A1 - Rochman, Dimitri A1 - Schillebeeckx, Peter A1 - Seidl, Marcus A1 - Hernandez Solis, Augusto A1 - Stankovskiy, Alexey A1 - Alvarez Velarde, Francisco A1 - Verwerft, Marc A1 - Rodriguez Villagra, Nieves A1 - Wiss, Thierry A1 - Zencker, Uwe A1 - Žerovnik, Gasper T1 - EURAD Work Package 8 Deliverable 8.2 Updated State-of-the-Art Report N2 - The state-of-the-art (SOTA) report offers an overview of the status of knowledge in the area of spent nuclear fuel (SNF) characterisation and assessment during the pre-disposal phase using several numerical and experimental approaches and methodologies. A review on characterisation of SNF properties in terms of source term and inventory assessment (neutron, gamma-ray emission, decay heat, radionuclide inventory, and elemental content) and in terms of out-of-core fuel performance (cladding performance and fuel integrity in view of the safety criteria for SNF interim storage, transport and canister packaging) is presented. This updated SOTA report provides the progress made in the spent fuel characterisation (SFC) work package as part of the European Joint Programme on Radioactive Waste Management (EURAD), documents the identified technical gaps, and provides recommendations for future work. The report is expected to be used by all EURAD colleagues in their national programmes as a key resource for knowledge management programmes and to contribute to demonstrating and documenting the state-of-the-art. KW - Radioactive waste management KW - Spent fuel characterisation KW - Extended interim storage KW - Predisposal PY - 2024 UR - https://www.ejp-eurad.eu/publications/d82-updated-state-art-report SP - 1 EP - 182 AN - OPUS4-61218 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - CONF A1 - Weber, Mike A1 - Völzke, Holger A1 - Zencker, Uwe A1 - Hauer, Katharina A1 - Herz, A. A1 - Kreienmeyer, M. T1 - Aufbau eines Aufprallfundamentes mit reproduzierbaren Eigenschaften für Baumusterprüfungen von Abfallbehältern für das Endlager Konrad N2 - Abgeleitet aus den in Teil 3 der „Systemanalyse Konrad“ definierten Lastannahmen für den „untertägigen Anlagenbereich“ müssen Verpackungen, die der Abfallbehälterklasse I (ABK I) mit dem zusätzlichen Merkmal der störfallfesten (sf) Verpackung oder der ABK II zugeordnet werden, gemäß den „Endlagerungsbedingungen, Endlager Konrad“, nach einem „…Fall aus 5 m Höhe auf eine unnachgiebige Unterlage…“ bestimmten Anforderungen genügen. Eine nähere Beschreibung der Prüfeinrichtung sowie die Definition detaillierter Anforderungen an das Aufprallfundament erfolgen in der „Produktkontrolle, Endlager Konrad“: „Die Prüfeinrichtung, bestehend aus einer Hebeeinrichtung und einem Fundament ist so zu gestalten, dass der Fall des Prüfmusters in jeder beliebigen Aufprallorientierung aus 5 m Höhe, gemessen von der Unterkante des Prüfmusters zum Fundament, möglich ist. Das Fundament ist aus Beton der Mindestgüte B 35 herzustellen und muss so beschaffen und verankert sein, dass keine Zerstörung in zahlreiche kleinere Bruchstücke erfolgt und keine horizontale Verschiebung des Fundamentes oder seiner Teile auftritt. Maße und Masse des Fundaments müssen so beschaffen sein, dass der Einfluss des Baugrundes unter dem Fundament auf den Aufprallwiderstand vernachlässigbar ist.“ Im Rahmen der Bauartprüfung für Behälter zur Endlagerung radioaktiver Abfälle mit zu vernachlässigender Wärmeentwicklung im Endlager Konrad wird die Bundesanstalt für Materialforschung und -prüfung (BAM) von der Bundesgesellschaft für Endlagerung (BGE) als Sachverständige hinzugezogen und ist in der Regel auch mit der Durchführung der notwendigen Fallprüfungen auf dem Testgelände Technische Sicherheit der BAM (BAM TTS) einschließlich der Bereitstellung der benötigten Prüfeinrichtungen sowie des regelkonformen Aufprallfundamentes beauftragt. Der Prozess, beginnend von der Gewährleistung einer von allen Beteiligten als gültig bewerteten Fallprüfung bis hin zur abschließenden Bewertung und Interpretation der Versuchsergebnisse erfordert dabei u.a. eine sorgfältige Planung und Fertigung der für das Endlager Konrad repräsentativen Fundamentplatte und deren Ankopplung an einen Untergrund im Sinne der „Regulations for the Safe Transport of Radioactive Material“ wie er zum Beispiel auf den beiden Fallversuchsanlagen des BAM Testgelände Technische Sicherheit (BAM TTS) zur Verfügung steht. Um diese Anforderungen zu erfüllen muss zum einen der Erhalt der Integrität der Fundamentplatte beim Fallversuch durch eine geeignete Auswahl und kraftflussgerechte Anordnung der Stabstahl-Bewehrung sowie deren Verankerung garantiert und damit eine unzulässige Energieaufnahme durch Risse sowie eine unzulässige „… Zerstörung (der Fundamentplatte) in zahlreiche kleinere Bruchstücke …“, wie in [3] gefordert, verhindert werden. Außerdem ist zu gewährleisten, dass der Beton die Anforderungen an die vorgeschriebene Mindestgüte bzw. -festigkeit zum Zeitpunkt der Fallprüfung erfüllt, die Betonfestigkeit jedoch zur Vermeidung unnötig verschärfter Prüfrandbedingungen eine zu definierende Obergrenze nicht überschreitet. Ausgehend von dem 2009 im Rahmen der KONTEC veröffentlichten Wissensstand präsentiert die BAM im vorliegenden Beitrag die wesentlichen Ergebnisse der zwischenzeitlich bei der Planung und Durchführung von zahlreichen Fallprüfungen gewonnenen Erfahrungen bzgl. Spezifikation und Fertigung der für die Fallversuche notwendigen Fundamentplatten sowie deren Anbindung an den Untergrund. Neben den immer wieder notwendigen Anstrengungen zur Gewährleistung einer im Rahmen der Definition korrekten Betondruckfestigkeit am Tag der Fallprüfung wird die Anpassung der Bewehrungsführung an verschiedene Fallpositionen diskutiert. Zur Ergänzung des gültigen Regelwerks entsteht parallel zu diesem Dokument eine Fachnotiz, in der BGE und BAM die Vorgaben und Spezifikationen zur regelwerkskonformen Herstellung und Montage von Fundamentplatten für Fallprüfungen im Rahmen der Behälterbauartprüfungsverfahren für das Endlager Konrad zusammenfassen und veröffentlichen werden. Diese Fachnotiz soll detaillierte Vorgaben und Spezifikationen zur Planung, Beauftragung, Herstellung und abschließenden Prüfung eines solchen Fundamentes und dessen Anbindung an den Untergrund enthalten. Damit soll allen beteiligten Organisationen wie Antragstellern, Sachverständigen und BGE ein langfristig verlässlicher Leitfaden im Hinblick auf die Durchführung anforderungsgerechter Fallprüfungen unter definierten und reproduzierbaren Randbedingungen im Rahmen der Bauartprüfungsverfahren für das Endlager Konrad an die Hand gegeben werden. T2 - KONTEC 2021 CY - Dresden, Germany DA - 25.08.2021 KW - Aufprallfundament KW - Endlager Konrad KW - Fallprüfung PY - 2021 SP - 1 EP - 10 CY - Dresden AN - OPUS4-53372 LA - deu AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - CONF A1 - Weber, Mike A1 - Völzke, Holger A1 - Zencker, Uwe A1 - Hauer, Katharina A1 - Herz, A. A1 - Kreienmeyer, M. T1 - Aufbau eines Aufprallfundamentes mit reproduzierbaren Eigenschaften für Baumusterprüfungen von Abfallbehältern für das Endlager Konrad N2 - Abgeleitet aus den in Teil 3 der „Systemanalyse Konrad“ [1] definierten Lastannahmen für den „untertägigen Anlagenbereich“ müssen Verpackungen, die der Abfallbehälterklasse I (ABK I) mit dem zusätzlichen Merkmal der störfallfesten (sf) Verpackung oder der ABK II zugeordnet werden, gemäß den „Endlagerungsbedingungen, Endlager Konrad“ [2], nach einem „…Fall aus 5 m Höhe auf eine unnachgiebige Unterlage…“ bestimmten Anforderungen genügen. Eine nähere Beschreibung der Prüfeinrichtung sowie die Definition detaillierter Anforderungen an das Aufprallfundament erfolgen in der „Produktkontrolle, Endlager Konrad“ [3]: „Die Prüfeinrichtung, bestehend aus einer Hebeeinrichtung und einem Fundament ist so zu gestalten, dass der Fall des Prüfmusters in jeder beliebigen Aufprallorientierung aus 5 m Höhe, gemessen von der Unterkante des Prüfmusters zum Fundament, möglich ist. Das Fundament ist aus Beton der Mindestgüte B 35 herzustellen und muss so beschaffen und verankert sein, dass keine Zerstörung in zahlreiche kleinere Bruchstücke erfolgt und keine horizontale Verschiebung des Fundamentes oder seiner Teile auftritt. Maße und Masse des Fundaments müssen so beschaffen sein, dass der Einfluss des Baugrundes unter dem Fundament auf den Aufprallwiderstand vernachlässigbar ist.“ Im Rahmen der Bauartprüfung für Behälter zur Endlagerung radioaktiver Abfälle mit zu vernachlässigender Wärmeentwicklung im Endlager Konrad wird die Bundesanstalt für Materialforschung und -prüfung (BAM) von der Bundesgesellschaft für Endlagerung (BGE) als Sachverständige hinzugezogen und ist in der Regel auch mit der Durchführung der notwendigen Fallprüfungen auf dem Testgelände Technische Sicherheit der BAM (BAM TTS) einschließlich der Bereitstellung der benötigten Prüfeinrichtungen sowie des regelkonformen Aufprallfundamentes beauftragt. Der Prozess, beginnend von der Gewährleistung einer von allen Beteiligten als gültig bewerteten Fallprüfung bis hin zur abschließenden Bewertung und Interpretation der Versuchsergebnisse erfordert dabei u.a. eine sorgfältige Planung und Fertigung der für das Endlager Konrad repräsentativen Fundamentplatte und deren Ankopplung an einen Untergrund im Sinne der „Regulations for the Safe Transport of Radioactive Material“ [4], [5] wie er zum Beispiel auf den beiden Fallversuchsanlagen des BAM Testgelände Technische Sicherheit (BAM TTS) zur Verfügung steht. Um diese Anforderungen zu erfüllen muss zum einen der Erhalt der Integrität der Fundamentplatte beim Fallversuch durch eine geeignete Auswahl und kraftflussgerechte Anordnung der Stabstahl-Bewehrung sowie deren Verankerung garantiert und damit eine unzulässige Energieaufnahme durch Risse sowie eine unzulässige „… Zerstörung (der Fundamentplatte) in zahlreiche kleinere Bruchstücke …“, wie in [3] gefordert, verhindert werden. Außerdem ist zu gewährleisten, dass der Beton die Anforderungen an die vorgeschriebene Mindestgüte bzw. -festigkeit zum Zeitpunkt der Fallprüfung erfüllt, die Betonfestigkeit jedoch zur Vermeidung unnötig verschärfter Prüfrandbedingungen eine zu definierende Obergrenze nicht überschreitet. Ausgehend von dem 2009 im Rahmen der KONTEC veröffentlichten Wissensstand [6] präsentiert die BAM im vorliegenden Beitrag die wesentlichen Ergebnisse der zwischenzeitlich bei der Planung und Durchführung von zahlreichen Fallprüfungen gewonnenen Erfahrungen bzgl. Spezifikation und Fertigung der für die Fallversuche notwendigen Fundamentplatten sowie deren Anbindung an den Untergrund. Neben den immer wieder notwendigen Anstrengungen zur Gewährleistung einer im Rahmen der Definition korrekten Betondruckfestigkeit am Tag der Fallprüfung wird die Anpassung der Bewehrungsführung an verschiedene Fallpositionen diskutiert. Zur Ergänzung des gültigen Regelwerks entsteht parallel zu diesem Dokument eine Fachnotiz, in der BGE und BAM die Vorgaben und Spezifikationen zur regelwerkskonformen Herstellung und Montage von Fundamentplatten für Fallprüfungen im Rahmen der Behälterbauartprüfungsverfahren für das Endlager Konrad zusammenfassen und veröffentlichen werden. Diese Fachnotiz soll detaillierte Vorgaben und Spezifikationen zur Planung, Beauftragung, Herstellung und abschließenden Prüfung eines solchen Fundamentes und dessen Anbindung an den Untergrund enthalten. Damit soll allen beteiligten Organisationen wie Antragstellern, Sachverständigen und BGE ein langfristig verlässlicher Leitfaden im Hinblick auf die Durchführung anforderungsgerechter Fallprüfungen unter definierten und reproduzierbaren Randbedingungen im Rahmen der Bauartprüfungsverfahren für das Endlager Konrad an die Hand gegeben werden. T2 - KONTEC 2021 CY - Dresden, Germany DA - 25.08.2021 KW - Endlager Konrad KW - Fallprüfung KW - Aufprallfundament PY - 2021 AN - OPUS4-53374 LA - deu AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - CONF A1 - Weber, Mike A1 - Völzke, Holger A1 - Zencker, Uwe A1 - Herz, A. A1 - Kreienmeyer, M. T1 - Design of a Drop Test Target with Reproducible Properties for Konrad Prototype Testing N2 - Beginning in 1976 the former iron ore mine Konrad was geologically investigated concerning its suitability as a location for a German final repository for low and intermediate level waste. After a comprehensive licensing procedure it was approved and is now being prepared and equipped for the planned start of storage in 2027. At the end of the 1980s, the requirements for waste containers for storage in this repository were defined for the first time on the basis of an incident analysis of the on-site handling procedures, beginning with the unloading of the packages after the arrival at the site up to the final positioning in the underground storage galleries. A 5-meter drop onto the rock ground of the mine was identified as the covering case for high mechanical requirements (ABK II container class). In contrast to the 9-meter drop according to the IAEA Regulations for the Safe Transport of Radioactive Material, the 5-meter drop is performed onto a hard but not essentially unyielding target. The container is typically not protected by an impact limiter. The requirements for a potential test facility are described in the regulations for the Konrad repository. The mechanical strength of the target is defined as a concrete strength equivalent to the identified properties of the rock ground of the mine. Since 1991 BAM has consistently used precast reinforced concrete slabs as target for drop tests in the framework of licensing procedures as well as in research projects. While the original design fulfilled the requirement for the integrity of the concrete slab in most cases, it failed when drop tests onto an edge of a container were performed. A redesigned concrete slab developed in a research project and suggested as a reference target in 2009 has been successfully used in Konrad licensing procedures since then. The paper gives a brief overview of the historical development and it describes BAM’s efforts and approaches to continuously guarantee a concrete slab of defined quality and to provide a test setup for valid drop tests from the applicants and the authorities view. T2 - PATRAM 2022, 20th International Symposium on the Packaging and Transportation of Radioactive Materials CY - Juan-les-Pins, France DA - 11.06.2023 KW - Target KW - Drop test KW - Final repository Konrad PY - 2023 SP - 1 EP - 11 AN - OPUS4-58563 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - CONF A1 - Zencker, Uwe T1 - EURAD WP 8 (SFC) - Task 3: Behaviour of nuclear fuel and cladding after discharge N2 - The European Joint Programme on Radioactive Waste Management (EURAD) deals in work package (WP) 8 with Spent Fuel Characterization (SFC). Inspired by the EURAD activities, an international Coordinated Research Project (CRP) on SFC was established by the International Atomic Energy Agency (IAEA). The EURAD WP SFC participants are collaborating as a team on the IAEA CRP on SFC. The EURAD WP SFC project is divided into four tasks. Task 3 investigates the behaviour of nuclear fuel and cladding after discharge. The aim of these activities is to understand and describe the evolution of the cladding-pellet system and its ageing under conditions of extended interim storage, transportation and emplacement in a final disposal system. During an IAEA consultancy meeting, BAM as leader of Task 3 reported on the current status of the research work. T2 - IAEA Consultancy Meeting on the Coordinated Research Project on Spent Fuel Characterization CY - Online meeting DA - 28.06.2021 KW - Nuclear Fuel KW - Cladding KW - Spent Fuel Characterization KW - Extended Interim Storage KW - Final Disposal PY - 2021 AN - OPUS4-52909 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - CONF A1 - Zencker, Uwe T1 - Fracture Mechanics Analysis of Spent Fuel Claddings during Long-Term Dry Interim Storage N2 - The prevention of brittle fracture of spent fuel claddings during long-term dry interim storage is based on experimental investigations, numerical analyses and assessment methods for predicting the mechanical behavior and determining limiting conditions. The ring compression test (RCT) is an established experimental method for characterizing cladding material. Test results for various high-burnup pressure water reactor zirconium-based fuel cladding alloys (e.g., ZIRLO®, M5®) are publicly available. To reduce the effort associated with irradiated samples in hot cells, it is helpful to perform studies on unirradiated surrogate cladding material. Based on such experimental data, load-displacement curves were numerically analyzed for selected cladding materials. In the presence of radial hydrides, a sample may suddenly fail by fracture even at small deformations. Noticeable load drops in the RCT occur associated to unstable crack propagation through the radial hydride network. The failure mechanism is quasi-cleavage in the hydrides and micro-void nucleation, growth, and coalescence in the zirconium matrix, with ductile tearing patches connecting neighboring hydrides. The failure process was simulated by cohesive zones controlled by the fracture energy and the cohesive strength. A modeling approach is presented in which the radial hydride morphology is taken into account. Based on the developed fracture mechanics approach with cohesive zone modeling, not only the deformation behavior but also the failure behavior of irradiated as well as unirradiated claddings with radial hydrides under RCT loading conditions can be adequately described. T2 - 20th International Symposium on the Packaging and Transportation of Radioactive Materials (PATRAM 2022) CY - Juan-les-Pins, France DA - 11.06.2023 KW - Extended Interim Storage KW - Nuclear Fuel Cladding KW - Numerical Failure Analysis KW - Ring Compression Test KW - Spent Fuel Characterization PY - 2023 AN - OPUS4-59147 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - CONF A1 - Zencker, Uwe T1 - EURAD WP 8 Task 3 Overview: Behaviour of nuclear fuel and cladding after discharge N2 - Task 3 of Work package 8 (Spent Fuel Characterization) of the European Joint Programme on Radioactive Waste Management (EURAD) investigates the behaviour of nuclear fuel and cladding after discharge. The aim of the work is to understand and describe the be-haviour of spent nuclear fuel (SNF), irradiated cladding, fuel/cladding chemical interaction (FCCI) and ageing under conditions of extended interim storage, transportation and em-placement in a final disposal system. BAM contributes to the project as partner and leads Task 3. The presentation gives an overview of the project status, main achievements in experimental work and modelling studies, deviations from the plan, delays and challenges ahead. T2 - EURAD Work Package 8 (SFC) Annual Meeting CY - Wettingen, Switzerland DA - 31.10.2023 KW - Nuclear fuel KW - Cladding KW - Discharge PY - 2023 AN - OPUS4-59148 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - CONF A1 - Zencker, Uwe T1 - Spent Fuel Characterization - Current Activities at BAM N2 - The European Joint Programme on Radioactive Waste Management (EURAD) is working on Spent Fuel Characterization (SFC) in its work package (WP) 8. Inspired by the EURAD activities, the International Atomic Energy Agency (IAEA) established an international Coordinated Research Project (CRP) on SFC. The EURAD WP SFC participants are collaborating as a team on the IAEA CRP on SFC. The EURAD WP SFC project consists of four tasks. Task 3 investigates the behaviour of nuclear fuel and cladding after discharge. The aim of these activities is to understand and describe the evolution of the cladding-pellet system and its ageing under conditions of extended interim storage, transportation and emplacement in a final disposal system. At a Consultancy Meeting, BAM as contributor to Task 3 presented current results of the failure analysis of irradiated ZIRLO® claddings under conditions of the Ring Compression Test. T2 - IAEA Consultancy Meeting on the Coordinated Research Project on Spent Fuel Characterization CY - Online meeting DA - 12.09.2023 KW - Nuclear Fuel Cladding KW - Numerical Failure Analysis KW - Ring Compression Test KW - Spent Fuel Characterization KW - Extended Interim Storage PY - 2023 AN - OPUS4-58276 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - CONF A1 - Zencker, Uwe T1 - EURAD WP 8 Task 3 Overview: Behaviour of nuclear fuel and cladding after discharge N2 - Task 3 of Work package 8 (Spent Fuel Characterization) of the European Joint Programme on Radioactive Waste Management (EURAD) investigates the behaviour of nuclear fuel and cladding after discharge. The aim of the work is to understand and describe the behaviour of spent nuclear fuel (SNF), irradiated cladding, fuel/cladding chemical interaction (FCCI) and ageing under conditions of extended interim storage, transportation and emplacement in a final disposal system. BAM contributes to the project as partner and leads Task 3. The presentation gives an overview of the project status, main achievements in experimental work and modelling studies, deviations from the plan, delays and challenges ahead. T2 - EURAD Work Package 8 (SFC) Annual Meeting CY - Kalmar, Sweden DA - 19.09.2022 KW - Nuclear fuel KW - Cladding KW - Discharge PY - 2022 AN - OPUS4-56120 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - CONF A1 - Zencker, Uwe T1 - EURAD WP 8 (SFC) Task 3 - Update: Behaviour of nuclear fuel and cladding after discharge N2 - The European Joint Programme on Radioactive Waste Management (EURAD) is working on Spent Fuel Characterization (SFC) in its work package (WP) 8. Inspired by the EURAD activities, the International Atomic Energy Agency (IAEA) established an international Coordinated Research Project (CRP) on SFC. The EURAD WP SFC participants are collaborating as a team on the IAEA CRP on SFC. The EURAD WP SFC project consists of four tasks. Task 3 investigates the behaviour of nuclear fuel and cladding after discharge. The aim of these activities is to understand and describe the evolution of the cladding-pellet system and its ageing under conditions of extended interim storage, transportation and emplacement in a final disposal system. At the Second Research Coordination Meeting on Spent Fuel Characterization, BAM as leader of Task 3 reported on the status of the research work. T2 - IAEA 2nd Research Coordination Meeting of the Coordinated Research Project on Spent Fuel Characterization CY - Kalmar, Sweden DA - 20.09.2022 KW - Nuclear fuel KW - Cladding KW - Discharge PY - 2022 AN - OPUS4-56121 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - CONF A1 - Zencker, Uwe T1 - Brittle Failure Limits of Spent Fuel Claddings Subjected to Long-Term Dry Interim Storage Conditions N2 - The mechanical properties of spent fuel claddings can be adversely affected under the conditions of long-term dry interim storage, so that the failure limits may be reached in case of mechanical loads during handling or transport after storage. Pre-storage drying and the early stage of interim storage can expose the cladding to higher temperatures and higher tensile hoop stresses than those associated with in-reactor operation and pool storage. During slow cooling of a cladding tube under internal pressure, radial hydrides may precipitate in zirconium-based cladding alloys. This can lead to embrittlement of the material and sudden failure of the cladding integrity under mechanical stress. In order to prevent brittle failure, numerical methods are being developed to predict the mechanical behaviour and identify limiting conditions. Experimental investigations, numerical analyses and evaluation methods are discussed. An established experimental method for characterising cladding materials is the Ring Compression Test (RCT). Some test results on irradiated cladding tubes after operation in pressure water reactors are publicly available. However, it is helpful to carry out studies on unirradiated surrogate claddings with similar material properties to reduce the effort associated with irradiated samples in hot cells and to perform material tests with a wider range of parameters. On the basis of such experimental data, load-displacement curves have been numerically analysed for a selection of cladding materials. Radial hydrides can cause a sample to break suddenly due to fracture even at low deformation. Noticeable load drops in the RCT are caused by unstable crack propagation through the radial hydride network. The failure mechanism is quasi-cleavage in the hydrides and micro-void nucleation, growth, and coalescence in the zirconium matrix, with ductile tearing patches connecting adjacent hydrides. The cohesive zone approach was used to simulate the failure process taking into account the radial hydride morphology. The developed method can adequately describe both the deformation and failure behaviour of irradiated as well as unirradiated claddings of zirconium-based alloys with radial hydrides under RCT conditions. Limiting conditions can be expressed in terms of fracture energy and cohesive strength. T2 - IAEA International Conference on the Management of Spent Fuel from Nuclear Power Plants - Meeting the Moment CY - Vienna, Austria DA - 10.06.2024 KW - Ageing Management KW - Cladding Embrittlement KW - Extended Storage KW - Ring Compression Test KW - Spent Nuclear Fuel PY - 2024 AN - OPUS4-60324 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - CONF A1 - Zencker, Uwe T1 - Fracture Mechanics Analysis of Spent Fuel Claddings during Long-Term Dry Interim Storage N2 - The European Joint Programme on Radioactive Waste Management (EURAD) is working on Spent Fuel Characterization (SFC) in its work package (WP) 8. Inspired by the EURAD activities, the International Atomic Energy Agency (IAEA) established an international Coordinated Research Project (CRP) on SFC. The EURAD WP SFC participants are collaborating as a team on the IAEA CRP on SFC. The EURAD WP SFC project consists of four tasks. Task 3 investigates the behaviour of nuclear fuel and cladding after discharge. The aim of these activities is to understand and describe the evolution of the cladding-pellet system and its ageing under conditions of extended interim storage, transportation and emplacement in a final disposal system. At the Third Research Coordination Meeting on Spent Fuel Characterization, BAM as contributor to Task 3 reported on the activities and status of its research work. T2 - IAEA 3rd Research Coordination Meeting of the Coordinated Research Project on Spent Fuel Characterization CY - Cockermouth, UK DA - 01.07.2024 KW - Nuclear fuel KW - Cladding KW - Discharge PY - 2024 AN - OPUS4-60668 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - CONF A1 - Zencker, Uwe T1 - Failure Analysis on Irradiated Claddings Subjected to Long-Term Dry Interim Storage N2 - Long-term dry interim storage may adversely affect the mechanical properties of spent fuel rods, possibly resulting in a reduced resilience during handling or transport after storage. The cladding is the first barrier for the spent fuel pellets. An established method for characterising the cladding material is the ring compression test (RCT), in which a small, cylindrical sample of the cladding tube is subjected to a compressive load. Radial hydrides may precipitate in zirconium-based alloys (Zircaloy) under pre-storage drying and during slow cooling, which result in embrittlement of the cladding material and eventually a possible sudden failure of cladding integrity under additional mechanical loads. The focus of the presented research is on the development of appropriate nu-merical methods for predicting the mechanical behaviour and identification of limiting conditions to prevent brittle fracture of Zircaloy claddings. A modelling approach based on cohesive zones is ex-plained which is able to reproduce the propagation of cracks initiated at radial hydrides in the zir-conium matrix. The developed methods are applied to defueled samples of cladding alloy ZIRLO®, which were subjected to a thermo-mechanical treatment to reorient existing circumferential hy-drides to radial hydrides. A selected sample showing sudden load drops during a quasi-static ring compression test is analysed by means of fracture mechanics for illustrative purposes. Based on the developed fracture mechanics approach, not only the deformation behaviour but also the fail-ure behaviour of irradiated as well as unirradiated Zircaloy claddings with radial hydrides under RCT loading conditions can be adequately described. T2 - 27th International Conference on Structural Mechanics in Reactor Technology - SMiRT 27 CY - Yokohama, Japan DA - 03.03.2024 KW - Cladding Embrittlement KW - Cohesive Zone Modelling KW - Ring Compression Test KW - Spent Nuclear Fuel PY - 2024 AN - OPUS4-60672 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - CONF A1 - Zencker, Uwe T1 - Analysis of Zirconium Hydride Structures in Spent Fuel Claddings Subjected to Storage Conditions N2 - Pre-storage drying and the early stage of storage can subject spent fuel claddings to higher temperatures and higher tensile hoop stresses than those associated with in-reactor operation. Under these conditions, existing circumferential hydrides in zirconium-based alloys can be partly reoriented into radial ones that may result in embrittlement of the cladding material. As a consequence, the failure limits may be reduced under mechanical loads caused by handling or during transport after storage. The potential occurrence of brittle fracture strongly depends on the specific location, size, and orientation of the zirconium hydrides. The morphology of such hydride structures was experimentally investigated in unirradiated, hydrogen-loaded samples made of a zirconium-based alloy. The hydrogen was introduced into the cladding sample by means of a cathodic charging process. The loading process was followed by a thermal treatment to precipitate the hydrides in the circumferential direction and then a thermomechanical treatment to reorient the hydrides in the radial direction. Metallographic methods were used to describe and classify the hydride morphology. The resulting metallographic micrographs were evaluated using suitable radial hydride metrics. The determination of the maximum length of a hydride structure was carried out in two different ways, each with its own advantages and disadvantages. Both methods consider neighboring hydrides as continuous according to the definition of the Radial Hydride Continuity Factor (RHCF). The first option is to measure the Euclidean distance between the two most distant pixels of the hydride structure in the image analysis, whereby the actual maximum size of the hydride structure is determined. The second possibility is to measure the maximum size of a hydride or a hydride structure within a certain arc length in the radial direction of the cladding tube. This value is of particular interest because the ratio of the maximum radial size of a hydride structure to the wall thickness of the cladding tube is used for the safety assessment of spent fuel claddings with radial hydrides using the RHCF. T2 - 21st International Symposium on the Packaging and Transportation of Radioactive Materials - PATRAM 2025 CY - San Antonio, TX, USA DA - 27.07.2025 KW - Extended Interim Storage KW - Nuclear Fuel Cladding KW - Zirconium Hydride Structure KW - Ring Compression Test KW - Micrograph Analysis PY - 2025 AN - OPUS4-63876 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - CONF A1 - Zencker, Uwe T1 - Failure Analysis on Spent Fuel Claddings Subjected to Long-Term Dry Interim Storage N2 - Long-term dry interim storage may adversely affect the mechanical properties of spent fuel claddings, possibly resulting in a reduced resilience during handling or transport after storage. Pre-storage drying and the early stage of interim storage can subject the cladding to higher temperatures and higher tensile hoop stresses than those associated with in-reactor operation and pool storage. Under these conditions, radial hydrides may precipitate in zirconium-based alloys (Zircaloy) during slow cooling, which result in embrittlement of the cladding material and eventually a possible sudden failure of cladding integrity under additional mechanical loads. Especially long, continuous radial hydride structures and low temperature can cause severe embrittlement of claddings and finally failure by fracture even at small deformations. Therefore, the study of hydride morphology plays an important role in describing the brittle failure behaviour of the claddings. The focus of the presented research is on the development of appropriate numerical methods for predicting the mechanical behaviour and identification of limiting conditions to prevent brittle fracture of Zircaloy claddings. An established experimental method for characterising cladding materials is the Ring Compression Test (RCT). Some test results on irradiated cladding tubes after operation in pressure water reactors are publicly available. However, it is helpful to carry out studies on unirradiated surrogate claddings with similar material properties to reduce the effort associated with irradiated samples in hot cells and to perform material tests with a wider range of parameters. On the basis of such experimental data, load-displacement curves have been numerically analysed for a selection of cladding materials. Radial hydrides can cause a sample to break suddenly. Noticeable load drops in the RCT are caused by unstable crack propagation through the radial hydride network. The failure mechanism is quasi-cleavage in the hydrides and micro-void nucleation, growth, and coalescence in the zirconium matrix, with ductile tearing patches connecting adjacent hydrides. The cohesive zone approach was used to simulate the failure process taking into account the radial hydride morphology. Experimental investigations, numerical analyses and evaluation methods for both the deformation and failure behaviour of irradiated as well as unirradiated claddings of zirconium-based alloys with radial hydrides are discussed. Limiting conditions can be expressed in terms of fracture energy and cohesive strength. T2 - IAEA Technical Meeting on the Behaviour of Spent Fuel and Cladding During Storage and the Performance of Spent Fuel Storage Systems CY - Seoul, South Korea DA - 23.06.2025 KW - Extended Interim Storage KW - Nuclear Fuel Cladding KW - Numerical Failure Analysis KW - Ring Compression Test KW - Spent Fuel Characterization PY - 2025 AN - OPUS4-63597 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - RPRT A1 - Zencker, Uwe A1 - Aguado, Carlos A1 - Arkoma, Asko A1 - Bertsch, Johannes A1 - Cristóbal Beneyto, Miguel A1 - Feria Marquez, Francisco A1 - Herranz, Luis Enrique A1 - Ivanov, Ivan A1 - Király, Márton A1 - Nasyrow, Ramil A1 - Papaioannou, Dimitrios A1 - Ruiz-Hervias, Jesus A1 - Vlassopoulos, Efstathios T1 - Thermo-mechanical-chemical properties of unirradiated and irradiated samples of spent nuclear fuel rod segments and cladding N2 - The report addresses the experimental characterisation, thermo-mechanical modelling and performance of unirradiated and irradiated samples of spent nuclear fuel rod segments and cladding. Hydrogen is relocated in nuclear fuel claddings by diffusion along temperature, stress, and concentration gradients, and towards a liner if existent. The precipitation of hydrides during cool-down at the beginning of the storage is influenced by mechanical stress. A strong accumulation of hydrides and a disadvantageous hydride alignment in relation to the stress state can affect the mechanical properties and compromise the fuel cladding integrity. Neutron radiography is used to determine spatially resolved hydrogen and hydride distributions in claddings. A liner in duplex claddings attracts hydrogen, which will then no longer be available to form detrimental hydrides in the bulk part of the cladding. Individual three-point bending and gravitational impact tests on filled pressurised spent nuclear fuel rod segments were conducted in hot-cell facilities. The material behaviour under three-point bending in the presence of hydrides and at different temperatures was systematically investigated in quasi-static laboratory tests on unirradiated rod segments with and without surrogate pellets until rupture. Ring compression tests were carried out on irradiated and unirradiated samples at different temperatures and both with and without radial hydrides. With radial hydrides, brittle failure is possible even at low deformation and simultaneously low temperature. Crack initiation will occur on the radial hydride with the highest fracture mechanics load, which depends on the hydride size in the regions with the highest hoop stresses. Due to the high hydrogen content used in creep tests conducted, precipitation hardening of the hydrides in the zirconium alloy significantly reduces the creep rate, as it strengthens the material and inhibits the dislocation sliding. The use of finite element analyses on mechanical tests to determine the cladding properties using a numerical optimisation method based on a large number of automatically generated sensitivity calculations is demonstrated. The brittle fracture of cladding samples with radial hydrides in the ring compression test can be described with a cohesive zone model if the cohesive parameters are selected appropriately and the hydride morphology is specified. Progress was made in the verification, validation and enhancement of spent fuel performance codes by the compilation of a representative validation database (related to rod internal pressure, fission gas release, rod void volume, and in-clad hydrogen distribution), the enhancement of CIEMAT’s FRAPCON-xt code for rod internal pressure prediction at high burnup, the enhancement of CIEMAT’s in-clad hydrogen performance subroutine HYDCLAD with more phenomenological modelling, the extension of INL’s BISON code with a cladding creep law for dry storage, and a benchmark with FRAPCON-xt and BISON simulating in-reactor and dry storage scenarios. KW - Spent Nuclear Fuel KW - Cladding KW - Experimental Characterisation KW - Modelling KW - Fuel Performance Code PY - 2024 SP - 1 EP - 102 PB - European Joint Programme EURAD AN - OPUS4-61008 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - CONF A1 - Zencker, Uwe A1 - Gaddampally, Mohan Reddy A1 - Völzke, Holger T1 - Fracture Mechanics Analysis of Spent Fuel Claddings during Long-Term Dry Interim Storage N2 - The prevention of brittle fracture of spent fuel claddings during long-term dry interim storage is based on experimental investigations, numerical analyses and assessment methods for predicting the mechanical behavior and determining limiting conditions. The ring compression test (RCT) is an established experimental method for characterizing cladding material. Test results for various high-burnup pressure water reactor zirconium-based fuel cladding alloys (e.g., ZIRLO®, M5®) are publicly available. To reduce the effort associated with irradiated samples in hot cells, it is helpful to perform studies on unirradiated surrogate cladding material. Based on such experimental data, load-displacement curves were numerically analyzed for selected cladding materials. In the presence of radial hydrides, a sample may suddenly fail by fracture even at small deformations. Noticeable load drops in the RCT occur associated to unstable crack propagation through the radial hydride network. The failure mechanism is quasi-cleavage in the hydrides and micro-void nucleation, growth, and coalescence in the zirconium matrix, with ductile tearing patches connecting neighboring hydrides. The failure process was simulated by cohesive zones controlled by the fracture energy and the cohesive strength. A modeling approach is presented in which the radial hydride morphology is taken into account. Based on the developed fracture mechanics approach with cohesive zone modeling, not only the deformation behavior but also the failure behavior of irradiated as well as unirradiated claddings with radial hydrides under RCT loading conditions can be adequately described. T2 - 20th International Symposium on the Packaging and Transportation of Radioactive Materials (PATRAM 2022) CY - Juan-les-Pins, France DA - 11.06.2023 KW - Extended Interim Storage KW - Nuclear Fuel Cladding KW - Numerical Failure Analysis KW - Ring Compression Test KW - Spent Fuel Characterization PY - 2023 SP - 1 EP - 8 AN - OPUS4-59146 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - CONF A1 - Zencker, Uwe A1 - Gaddampally, Mohan Reddy A1 - Völzke, Holger T1 - Failure Analysis on Irradiated Claddings Subjected to Long-Term Dry Interim Storage N2 - Long-term dry interim storage may adversely affect the mechanical properties of spent fuel rods, possibly resulting in a reduced resilience during handling or transport after storage. The cladding is the first barrier for the spent fuel pellets. An established method for characterising the cladding material is the ring compression test (RCT), in which a small, cylindrical sample of the cladding tube is subjected to a compressive load. Radial hydrides may precipitate in zirconium-based alloys (Zircaloy) under pre-storage drying and during slow cooling, which result in embrittlement of the cladding material and eventually a possible sudden failure of cladding integrity under additional mechanical loads. The focus of the presented research is on the development of appropriate nu-merical methods for predicting the mechanical behaviour and identification of limiting conditions to prevent brittle fracture of Zircaloy claddings. A modelling approach based on cohesive zones is ex-plained which is able to reproduce the propagation of cracks initiated at radial hydrides in the zir-conium matrix. The developed methods are applied to defueled samples of cladding alloy ZIRLO®, which were subjected to a thermo-mechanical treatment to reorient existing circumferential hy-drides to radial hydrides. A selected sample showing sudden load drops during a quasi-static ring compression test is analysed by means of fracture mechanics for illustrative purposes. Based on the developed fracture mechanics approach, not only the deformation behaviour but also the fail-ure behaviour of irradiated as well as unirradiated Zircaloy claddings with radial hydrides under RCT loading conditions can be adequately described. T2 - 27th International Conference on Structural Mechanics in Reactor Technology - SMiRT 27 CY - Yokohama, Japan DA - 03.03.2024 KW - Cladding Embrittlement KW - Cohesive Zone Modelling KW - Ring Compression Test KW - Spent Nuclear Fuel PY - 2024 SP - 1 EP - 8 AN - OPUS4-60671 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - RPRT A1 - Zencker, Uwe A1 - Simbruner, Kai A1 - Völzke, Holger T1 - Entwicklung eines bruchmechanischen Berechnungsansatzes zur Beschreibung des Festigkeitsverhaltens von Brennstabhüllrohren bei längerfristiger Zwischenlagerung (BRUZL) N2 - Es werden Methoden zur sicherheitstechnischen Bewertung des mechanischen Verhaltens von Brennstabhüllrohren entwickelt, um sprödes Versagen in Belastungsszenarien nach längerfristiger trockener Zwischenlagerung zu verhindern. Unbestrahlte Brennstabhüllrohrsegmente aus der Zirkoniumlegierung ZIRLO® wurden hydriert und thermomechanischen Behandlungen unterzogen, um Hüllrohrmaterial durch Ausscheidung radialer Hydride zu verspröden. Die Proben mit radialen Hydriden wurden im Ring Compression Test (RCT) bei Raumtemperatur untersucht. Bereits bei kleinen Probenverformungen wurden abrupte Kraftabfälle mit instabiler Rissausbreitung durch das Netzwerk radialer Hydride beobachtet. Die Risslängen erreichten in einigen Fällen bis zu 90 % der Wanddicke. Der mikromechanische Versagensmechanismus ist Quasi-Spaltbruch in den Hydriden und Porenbildung, -wachstum und -vereinigung in der Zirkoniummatrix an den duktilen Brücken zwischen benachbarten Hydriden. Es wurde ein Finite-Elemente-Modell des Ring Compression Tests erstellt, um das Versagensverhalten zirkoniumbasierter Legierungen mit radialen Hydriden im RCT zu analysieren. Die Fließkurve für das elastisch-plastische Materialmodell des Matrixmaterials wurde durch eine inverse Finite-Elemente-Analyse ermittelt. Kohäsivzonenmodelle wurden benutzt, um die plötzlichen Kraftabfälle zu reproduzieren. Es wurde ein mikromechanisches Modell mit statistisch generierten Matrix-Hydrid-Verteilungen entwickelt, das zwischen sprödem Versagen entlang der Hydride und duktilem Versagen der Zirkoniummatrix in der Kohäsivzone unterscheidet. Für das jeweilige Materialverhalten wird ein lokales zweiparametriges Versagenskriterium auf Grundlage der Kohäsionsfestigkeit und der Separationsenergie bei einer festgelegten Form des Kohäsivgesetzes vorgeschlagen. Geeignete Kohäsivparameter lassen sich mit einer inversen Finite-Elemente-Analyse des Versagensverhaltens von hydrierten Proben im Ring Compression Test bestimmen. In den Simulationen lag der Schwerpunkt auf dem ersten Kraftabfall. Die Berechnungsergebnisse stimmen gut mit den RCT-Ergebnissen überein. Es konnte gezeigt werden, dass die Rissinitiierung und -ausbreitung stark von der speziellen Anordnung der radialen Hydride und Matrixbrücken in der Bruchzone abhängt. Die numerische Modellbildung wurde an Versuchen mit bestrahlten Proben aus der Zirkoniumlegierung M5® validiert. KW - Zwischenlagerung KW - Brennstabhüllrohr KW - Versagensmechanismus KW - Kohäsivzonenmodell KW - Ring Compression Test PY - 2022 SP - 1 EP - 106 PB - Bundesanstalt für Materialforschung und -prüfung (BAM) CY - Berlin AN - OPUS4-56853 LA - deu AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - CONF A1 - Zencker, Uwe A1 - Simbruner, Kai A1 - Völzke, Holger T1 - Analysis of Zirconium Hydride Structures in Spent Fuel Claddings Subjected to Storage Conditions N2 - Pre-storage drying and the early stage of storage can subject spent fuel claddings to higher temperatures and higher tensile hoop stresses than those associated with in-reactor operation. Under these conditions, existing circumferential hydrides in zirconium-based alloys can be partly reoriented into radial ones that may result in embrittlement of the cladding material. As a consequence, the failure limits may be reduced under mechanical loads caused by handling or during transport after storage. The potential occurrence of brittle fracture strongly depends on the specific location, size, and orientation of the zirconium hydrides. The morphology of such hydride structures was experimentally investigated in unirradiated, hydrogen-loaded samples made of a zirconium-based alloy. The hydrogen was introduced into the cladding sample by means of a cathodic charging process. The loading process was followed by a thermal treatment to precipitate the hydrides in the circumferential direction and then a thermomechanical treatment to reorient the hydrides in the radial direction. Metallographic methods were used to describe and classify the hydride morphology. The resulting metallographic micrographs were evaluated using suitable radial hydride metrics. The determination of the maximum length of a hydride structure was carried out in two different ways, each with its own advantages and disadvantages. Both methods consider neighboring hydrides as continuous according to the definition of the Radial Hydride Continuity Factor (RHCF). The first option is to measure the Euclidean distance between the two most distant pixels of the hydride structure in the image analysis, whereby the actual maximum size of the hydride structure is determined. The second possibility is to measure the maximum size of a hydride or a hydride structure within a certain arc length in the radial direction of the cladding tube. This value is of particular interest because the ratio of the maximum radial size of a hydride structure to the wall thickness of the cladding tube is used for the safety assessment of spent fuel claddings with radial hydrides using the RHCF. T2 - 21st International Symposium on the Packaging and Transportation of Radioactive Materials - PATRAM 2025 CY - San Antonio, TX, USA DA - 27.07.2025 KW - Extended Interim Storage KW - Nuclear Fuel Cladding KW - Zirconium Hydride Structure KW - Ring Compression Test KW - Micrograph Analysis PY - 2025 SP - 1 EP - 8 CY - Indianapolis, IN, USA AN - OPUS4-63875 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER - TY - CONF A1 - Zencker, Uwe A1 - Völzke, Holger T1 - Brittle Failure Limits of Spent Fuel Claddings Subjected to Long-Term Dry Interim Storage Conditions N2 - The mechanical properties of spent fuel claddings can be adversely affected under the conditions of long-term dry interim storage, so that the failure limits may be reached in case of mechanical loads during handling or transport after storage. Pre-storage drying and the early stage of interim storage can expose the cladding to higher temperatures and higher tensile hoop stresses than those associated with in-reactor operation and pool storage. During slow cooling of a cladding tube under internal pressure, radial hydrides may precipitate in zirconium-based cladding alloys. This can lead to embrittlement of the material and sudden failure of the cladding integrity under mechanical stress. In order to prevent brittle failure, numerical methods are being developed to predict the mechanical behaviour and identify limiting conditions. Experimental investigations, numerical analyses and evaluation methods are discussed. An established experimental method for characterising cladding materials is the Ring Compression Test (RCT). Some test results on irradiated cladding tubes after operation in pressure water reactors are publicly available. However, it is helpful to carry out studies on unirradiated surrogate claddings with similar material properties to reduce the effort associated with irradiated samples in hot cells and to perform material tests with a wider range of parameters. On the basis of such experimental data, load-displacement curves have been numerically analysed for a selection of cladding materials. Radial hydrides can cause a sample to break suddenly due to fracture even at low deformation. Noticeable load drops in the RCT are caused by unstable crack propagation through the radial hydride network. The failure mechanism is quasi-cleavage in the hydrides and micro-void nucleation, growth, and coalescence in the zirconium matrix, with ductile tearing patches connecting adjacent hydrides. The cohesive zone approach was used to simulate the failure process taking into account the radial hydride morphology. The developed method can adequately describe both the deformation and failure behaviour of irradiated as well as unirradiated claddings of zirconium-based alloys with radial hydrides under RCT conditions. Limiting conditions can be expressed in terms of fracture energy and cohesive strength. T2 - IAEA International Conference on the Management of Spent Fuel from Nuclear Power Plants - Meeting the Moment CY - Vienna, Austria DA - 10.06.2024 KW - Ageing Management KW - Cladding Embrittlement KW - Extended Storage KW - Ring Compression Test KW - Spent Nuclear Fuel PY - 2024 SP - 1 EP - 10 AN - OPUS4-60323 LA - eng AD - Bundesanstalt fuer Materialforschung und -pruefung (BAM), Berlin, Germany ER -