Quantum control in size selected semiconductor quantum dot thin films

62585 2025 eng 229 239 2 14 article Walter de Gruyter GmbH 1 -- -- -- Quantum control in size selected semiconductor quantum dot thin films We introduce a novel technique for coherent control that employs resonant internally generated fields in CdTe quantum dot (QD) thin films at the L-point. The bulk band gap of CdTe at the L-point amounts to 3.6 eV, with the transition marked by strong Coulomb coupling. Third harmonic generation (λ3 = 343 nm, hν = 3.61 eV) for a fundamental wavelength of λ 1 = 1,030 nm is used to control quantum interference of three-photon resonant paths between the valence and conduction bands. Different thicknesses of the CdTe QDs are used to manipulate the phase relationship between the external fundamental and the internally generated third harmonic, resulting in either suppression or strong enhancement of the resonant third harmonic, while the nonresonant components remain nearly constant. This development could pave the way for new quantum interference–based applications in ultrafast switching of nanophotonic devices. Nanophotonics 10.1515/nanoph-2024-0529 urn:nbn:de:kobv:b43-625859 true {"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2025,2,9]],"date-time":"2025-02-09T05:14:03Z","timestamp":1739078043880,"version":"3.37.0"},"reference-count":59,"publisher":"Walter de Gruyter GmbH","issue":"2","license":[{"start":{"date-parts":[[2025,1,16]],"date-time":"2025-01-16T00:00:00Z","timestamp":1736985600000},"content-version":"unspecified","delay-in-days":0,"URL":"http:\/\/creativecommons.org\/licenses\/by\/4.0"}],"funder":[{"name":"Funda\u00e7\u00e3o de Amparo a Pesquisa do Estado de S\u00e3o Paulo in Brazil","award":["2021\/01170-3","2013\/07793-6"]},{"DOI":"10.13039\/501100001659","name":"Deutsche Forschungsgemeinschaft","doi-asserted-by":"publisher","award":["CRC1459","Za 110\/28 \u2013 1"],"id":[{"id":"10.13039\/501100001659","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2025,2,10]]},"abstract":"Abstract<\/jats:title>\n We introduce a novel technique for coherent control that employs resonant internally generated fields in CdTe quantum dot (QD) thin films at the L<\/jats:italic>-point. The bulk band gap of CdTe at the L<\/jats:italic>-point amounts to 3.6\u202feV, with the transition marked by strong Coulomb coupling. Third harmonic generation (\u03bb<\/jats:italic>\n 3<\/jats:sub> = 343\u202fnm, h\u03bd<\/jats:italic> = 3.61\u202feV) for a fundamental wavelength of \u03bb<\/jats:italic>\n 1<\/jats:sub> = 1,030\u202fnm is used to control quantum interference of three-photon resonant paths between the valence and conduction bands. Different thicknesses of the CdTe QDs are used to manipulate the phase relationship between the external fundamental and the internally generated third harmonic, resulting in either suppression or strong enhancement of the resonant third harmonic, while the nonresonant components remain nearly constant. This development could pave the way for new quantum interference\u2013based applications in ultrafast switching of nanophotonic devices.<\/jats:p>","DOI":"10.1515\/nanoph-2024-0529","type":"journal-article","created":{"date-parts":[[2025,1,15]],"date-time":"2025-01-15T17:20:43Z","timestamp":1736961643000},"page":"229-239","source":"Crossref","is-referenced-by-count":0,"title":["Quantum control in size selected semiconductor quantum dot thin films"],"prefix":"10.1515","volume":"14","author":[{"ORCID":"https:\/\/orcid.org\/0009-0002-1622-9857","authenticated-orcid":false,"given":"Victor","family":"K\u00e4rcher","sequence":"first","affiliation":[{"name":"Center for Soft Nanoscience , University of M\u00fcnster , 48149 M\u00fcnster , Germany"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-8720-5882","authenticated-orcid":false,"given":"Tobias","family":"Reiker","sequence":"additional","affiliation":[{"name":"Center for Soft Nanoscience , University of M\u00fcnster , 48149 M\u00fcnster , Germany"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4600-7817","authenticated-orcid":false,"given":"Pedro F.G.M.","family":"da Costa","sequence":"additional","affiliation":[{"name":"S\u00e3o Carlos Institute of Physics, University of S\u00e3o Paulo , S\u00e3o Carlos , SP 13566-590 , Brazil"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-8352-2573","authenticated-orcid":false,"given":"Andrea S.S.","family":"de Camargo","sequence":"additional","affiliation":[{"name":"Federal Institute for Materials Research and Testing (BAM) , 12489 Berlin , Germany"},{"name":"Friedrich-Schiller University Jena (FSU) , 07743 Jena , Germany"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9807-1103","authenticated-orcid":false,"given":"Helmut","family":"Zacharias","sequence":"additional","affiliation":[{"name":"Center for Soft Nanoscience , University of M\u00fcnster , 48149 M\u00fcnster , Germany"}]}],"member":"374","published-online":{"date-parts":[[2025,1,16]]},"reference":[{"key":"2025020810463819517_j_nanoph-2024-0529_ref_001","doi-asserted-by":"crossref","unstructured":"D. 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