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    <title language="eng">Probing Laser‐Driven Structure Formation at Extreme Scales in Space and Time</title>
    <abstract language="eng">Irradiation of solid surfaces with high intensity, ultrashort laser pulses triggers a variety of secondary processes that can lead to the formation of transient and permanent structures over a large range of length scales from mm down to the nano‐range. One of the most prominent examples are LIPSS – Laser‐Induced Periodic Surface Structures. While LIPSS have been a scientific evergreen for of almost 60 years, experimental methods that combine ultrafast temporal with the required nm spatial resolution have become available only recently with the advent of short pulse, short wavelength free electron lasers. Here, the current status and future perspectives in this field are discussed by exploiting the unique possibilities of these 4th‐generation light sources to address by time‐domain experimental techniques the fundamental LIPSS‐question, namely why and how laser irradiation can initiate the transition of a “chaotic” (rough) surface from an aperiodic into a periodic structure.</abstract>
    <parentTitle language="eng">Laser &amp; Photonics Reviews</parentTitle>
    <identifier type="issn">1863-8899</identifier>
    <identifier type="doi">10.1002/lpor.202300912</identifier>
    <identifier type="urn">urn:nbn:de:kobv:b43-595048</identifier>
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One of the most prominent examples are LIPSS \u2013 Laser\u2010Induced Periodic Surface Structures. While LIPSS have been a scientific evergreen for of almost 60 years, experimental methods that combine ultrafast temporal with the required nm spatial resolution have become available only recently with the advent of short pulse, short wavelength free electron lasers. Here, the current status and future perspectives in this field are discussed by exploiting the unique possibilities of these 4th\u2010generation light sources to address by time\u2010domain experimental techniques the fundamental LIPSS\u2010question, namely why and how laser irradiation can initiate the transition of a \u201cchaotic\u201d (rough) surface from an aperiodic into a periodic structure.&lt;\/jats:p&gt;","DOI":"10.1002\/lpor.202300912","type":"journal-article","created":{"date-parts":[[2024,2,9]],"date-time":"2024-02-09T03:53:36Z","timestamp":1707450816000},"update-policy":"http:\/\/dx.doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Probing Laser\u2010Driven Structure Formation at Extreme Scales in Space and Time"],"prefix":"10.1002","author":[{"ORCID":"http:\/\/orcid.org\/0000-0003-4984-3896","authenticated-orcid":false,"given":"J\u00f6rn","family":"Bonse","sequence":"first","affiliation":[{"name":"Bundesanstalt f\u00fcr Materialforschung und \u2010pr\u00fcfung (BAM)  Unter den Eichen 87 D\u201012205 Berlin Germany"}]},{"ORCID":"http:\/\/orcid.org\/0000-0002-7979-5357","authenticated-orcid":false,"given":"Klaus","family":"Sokolowski\u2010Tinten","sequence":"additional","affiliation":[{"name":"Faculty of Physics and Centre for Nanointegration Duisburg\u2010Essen University of Duisburg\u2010Essen Lotharstrasse 1 D\u201047057 Duisburg Germany"}]}],"member":"311","published-online":{"date-parts":[[2024,2,8]]},"reference":[{"key":"e_1_2_6_1_1","doi-asserted-by":"crossref","volume":"46","author":"Fann W. 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    <licence>Creative Commons - CC BY - Namensnennung 4.0 International</licence>
    <author>Jörn Bonse</author>
    <author>Klaus Sokolowski‐Tinten</author>
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      <language>eng</language>
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      <value>Laser-induced periodic surface structures (LIPSS)</value>
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    <subject>
      <language>eng</language>
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      <value>Free electron laser</value>
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    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>Pump-probe experiments</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>Time-resolved scattering</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>Capillary waves</value>
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    <collection role="ddc" number="620">Ingenieurwissenschaften und zugeordnete Tätigkeiten</collection>
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    <title language="eng">Characterisation of thin layers of Polydopamine used as functional coatings in X-Ray optics</title>
    <abstract language="eng">Polydopamine (PDA) is a biological / biomimetic polymer which has spiked considerable interest in recent years. Its monomer is an important neurotransmitter and it is one of the strongest glues produced by biological organisms. Polydopamine is a candidate for several applications, mainly in the field of biology and medicine, but also - recently - for layer coatings with optical, electrical, and mechanical function.&#13;
&#13;
In this work, we investigate PDA layers intended as reflectivity enhancers for mirror surfaces in X-ray astronomical observatories. It has previously been shown, that such X-ray telescopes can be improved by a coating of PDA in the thickness range of several nm. Accurate thickness determination is required to monitor and optimise the coating process. We use spectroscopic ellipsometry to determine first the dielectric function of the polydopamine layers using model coatings of sufficient thickness. This data is then used to accurately determine the layer thickness of much thinner PDA layers. This study resulted in data on the thickness and dielectric function of PDA layers that could lead to a better understanding of the correlation of layer thickness and layer properties depending on the process parameters.</abstract>
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    <author>Andreas Hertwig</author>
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      <value>Ellipsometry</value>
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    <subject>
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      <value>Polydopamine</value>
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    <subject>
      <language>eng</language>
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      <value>Thin Polymer Layers</value>
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    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>X-Ray Reflectometry</value>
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    <subject>
      <language>eng</language>
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      <value>Biopolymers</value>
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  <doc>
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    <publishedYear>2024</publishedYear>
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    <title language="deu">Gefährdung durch Röntgenemission bei der UKP-Laser-Materialbearbeitung</title>
    <abstract language="deu">Der Vortrag gibt einen Überblick zu ultrakurzen Laserpulsen, der Ultrakurzpulslaser-Materialbearbeitung und der dabei ggf. auftretenden unerwünschten Röntgenstrahlung. Es wird die Laserbearbeitung von technischen und biologischen Materialien diskutiert. Schutzmöglichkeiten gegenüber der Röntgenstrahlung werden erörtert.</abstract>
    <enrichment key="eventName">Sonthofer Strahlenschutztage 2024</enrichment>
    <enrichment key="eventPlace">Sonthofen, Germany</enrichment>
    <enrichment key="eventStart">11.03.2024</enrichment>
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    <author>Jörg Krüger</author>
    <subject>
      <language>deu</language>
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      <value>Ultrakurzpulslaser</value>
    </subject>
    <subject>
      <language>deu</language>
      <type>uncontrolled</type>
      <value>Laser-induzierte Röntgenstrahlung</value>
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    <subject>
      <language>deu</language>
      <type>uncontrolled</type>
      <value>Materialbearbeitung</value>
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    <subject>
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      <value>Technische Materialien</value>
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    <subject>
      <language>deu</language>
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      <value>Biologische Anwendungen</value>
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    <collection role="ddc" number="620">Ingenieurwissenschaften und zugeordnete Tätigkeiten</collection>
    <collection role="institutes" number="">6 Materialchemie</collection>
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    <publisherName>Zenodo</publisherName>
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    <title language="eng">Trinamic TMCL IOC for exposing Trinamics motor controllers to EPICS CA</title>
    <abstract language="eng">Trinamic TMCL IOC is a Python package designed for controlling stepper motors connected to a Trinamic board using the TMCL language (all boards supported by PyTrinamic should now work, has been tested on the TMCM 6110 and the TMCM 6214). Since it is implementing the TMCL protocol, it should be easy to adapt to other Trinamic motor controller boards. This package assumes the motor controller is connected over a machine network via a network-to-serial converter, but the underlying PyTrinamic package allows for other connections too.&#13;
&#13;
This allows the control of attached motors via the EPICS Channel-Access virtual communications bus. If EPICS is not desired, plain Pythonic control via motion_control should also be possible. An example for this will be provided in the example.ipynb Jupyter notebook.&#13;
&#13;
This package leverages Caproto for EPICS IOCs and a modified PyTrinamic library for the motor board control, and interfaces between the two via an internal set of dataclasses. Configuration for the motors and boards are loaded from YAML files (see tests/testdata/example_config.yaml).&#13;
&#13;
The modifications to PyTrinamic involved extending their library with a socket interface. This was a minor modification that should eventually find its way into the official package (a pull request has been submitted).</abstract>
    <identifier type="doi">10.5281/zenodo.10792593</identifier>
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    <enrichment key="ScientificNote">Complete software package for exposing Trinamics motor controllers to the EPICS industrial control system's Channel Access (CA) ethernet-based communications bus.</enrichment>
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    <licence>Creative Commons - CC BY - Namensnennung 4.0 International</licence>
    <author>Brian Richard Pauw</author>
    <subject>
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      <value>Instrumentation</value>
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    <subject>
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      <value>EPICS</value>
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      <value>Channel access</value>
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      <language>eng</language>
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      <value>Instrument control</value>
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    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>Laboratory automation</value>
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    <collection role="ddc" number="543">Analytische Chemie</collection>
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    <title language="deu">Röntgenstrahlungsexposition bei der Anwendung von Ultrakurzpulslasern in der Medizin</title>
    <abstract language="deu">Die Laserbearbeitung von Materialien mit ultrakurzen Laserpulsen kann zu einer sekundären Emission gefährlicher Röntgenstrahlen führen. Dieser Effekt wurde bisher bei der Bearbeitung von technischen Materialien wie Metallen beobachtet. Die Röntgenemission bei der abtragenden Bearbeitung von biologischen Geweben ist noch weitgehend unerforscht. Der Vortrag präsentiert erste Untersuchungen und Ergebnisse des radiologischen Gefährdungspotentials bei der medizinischen Anwendung von Ultrakurzpulslasern am Menschen.</abstract>
    <enrichment key="eventName">Bayerische Laserschutztage 2024</enrichment>
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    <author>Jörg Krüger</author>
    <subject>
      <language>deu</language>
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      <value>Ultrakurzpulslaser</value>
    </subject>
    <subject>
      <language>deu</language>
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      <value>Laser-induzierte Röntgenstrahlung</value>
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    <subject>
      <language>deu</language>
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      <value>Medizinische Anwendung</value>
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      <language>deu</language>
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      <value>Auge</value>
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    <subject>
      <language>deu</language>
      <type>uncontrolled</type>
      <value>Zahn</value>
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    <title language="eng">Base-pairing of uracil and 2,6-diaminopurine: from cocrystals to photoreactivity</title>
    <abstract language="eng">We show that the non-canonical nucleobase 2,6-diaminopurine (D) spontaneously base pairs with uracil (U) in water and the solid state without the need to be attached to the ribose-phosphate backbone. Depending on the reaction conditions, D and U assemble in thermodynamically stable hydrated and anhydrated D-U base-paired cocrystals. Under UV irradiation, an aqueous solution of D-U base-pair undergoes photochemical degradation, while a pure aqueous solution of U does not. Our simulations suggest that D may trigger the U photodimerization and show that complementary base-pairing modifies the photochemical properties of nucleobases, which might have implications for prebiotic chemistry.</abstract>
    <parentTitle language="eng">iScience</parentTitle>
    <identifier type="doi">10.1016/j.isci.2024.109894</identifier>
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    <author>Tomislav Stolar</author>
    <author>Ben K.D. Pearce</author>
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    <author>Luca Grisanti</author>
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      <value>In situ monitoring</value>
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      <value>Cocrystals</value>
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    <title language="eng">Mechanochemical Synthesis of a Sodium Anion Complex [Na&lt;sup&gt;+&lt;/sup&gt;(2,2,2-cryptand)Na&lt;sup&gt;–&lt;/sup&gt;] and Studies of Its Reactivity: Two-Electron and One-Electron Reductions</title>
    <abstract language="eng">Group 1 metal molecular chemistry is dominated by a +1 oxidation state, while a 0 oxidation state is widespread in the metals. A more exotic, yet still available, oxidation state of group 1 metal is −1, i.e., alkalide. Reported as early as the 1970s, the alkalides appear in every modern inorganic chemistry textbook as an iconic chemical curiosity, yet their reactivity remains unexplored. This is due to their synthetic hurdles. In this work, we report the first facile synthesis of the archetypical alkalide complex, [Na+(2,2,2-cryptand)Na–], which allows us to unveil a versatile reactivity profile of this once exotic species.</abstract>
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T.","key":"ref54\/cit54"},{"key":"ref55\/cit55","doi-asserted-by":"publisher","DOI":"10.1021\/ja00223a016"},{"key":"ref56\/cit56","doi-asserted-by":"publisher","DOI":"10.1002\/chem.202000194"}],"container-title":["Inorganic Chemistry"],"original-title":[],"language":"en","link":[{"URL":"https:\/\/pubs.acs.org\/doi\/pdf\/10.1021\/acs.inorgchem.4c02914","content-type":"application\/pdf","content-version":"vor","intended-application":"unspecified"},{"URL":"https:\/\/pubs.acs.org\/doi\/pdf\/10.1021\/acs.inorgchem.4c02914","content-type":"unspecified","content-version":"vor","intended-application":"similarity-checking"}],"deposited":{"date-parts":[[2024,8,12]],"date-time":"2024-08-12T07:29:18Z","timestamp":1723447758000},"score":1,"resource":{"primary":{"URL":"https:\/\/pubs.acs.org\/doi\/10.1021\/acs.inorgchem.4c02914"}},"subtitle":[],"short-title":[],"issued":{"date-parts":[[2024,7,29]]},"references-count":89,"journal-issue":{"issue":"32","published-print":{"date-parts":[[2024,8,12]]}},"alternative-id":["10.1021\/acs.inorgchem.4c02914"],"URL":"http:\/\/dx.doi.org\/10.1021\/acs.inorgchem.4c02914","relation":{},"ISSN":["0020-1669","1520-510X"],"issn-type":[{"type":"print","value":"0020-1669"},{"type":"electronic","value":"1520-510X"}],"subject":[],"published":{"date-parts":[[2024,7,29]]}}}</enrichment>
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    <licence>Creative Commons - CC BY - Namensnennung 4.0 International</licence>
    <author>Nathan Davison</author>
    <author>Jack M. Hemingway</author>
    <author>Corinne Wills</author>
    <author>Tomislav Stolar</author>
    <author>Paul G. Waddell</author>
    <author>Casey M. Dixon</author>
    <author>Luke Barron</author>
    <author>James A. Dawson</author>
    <author>Erli Lu</author>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>Mechanochemistry</value>
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    <language>eng</language>
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    <title language="eng">Ellipsometrical characterization of poly-dopamine layers considered for technical applications</title>
    <abstract language="eng">Although the organic molecule dopamine (3,4-dihydroxyphenethylamine) is commonly known as the “hormone of happiness”, thin films of poly-dopamine also have interesting technical properties. When produced by dip coating, the self-organizing layers grow in a reproducible thickness of single or multiple molecule monolayers of a few nanometer thickness only. In this work, we introduce a method of determining the layer thickness of poly-dopamine on mirrors for astronomical X-ray telescopes. This work is based on spectroscopic ellipsometry measurements and involves the development of an optical model for the poly-dopamine layers including the dielectric function. Thereby the complex refractive index of the produced layers was determined, covering the range from the ultraviolet to the near infrared spectral region. These measurement results and the corresponding technical challenges are presented in this contribution. Furthermore, an outlook to potential technical applications of this interesting material is given and poly-dopamine layers will make scientist and engineers hopefully happy as an innovative and fascinating technical solution for the future.</abstract>
    <parentTitle language="eng">Organic Electronics and Photonics: Fundamentals and Devices IV</parentTitle>
    <identifier type="doi">10.1117/12.3015281</identifier>
    <identifier type="isbn">978-1-5106-7344-1</identifier>
    <enrichment key="eventName">SPIE PHOTONICS EUROPE</enrichment>
    <enrichment key="eventPlace">Strasbourg. France</enrichment>
    <enrichment key="eventStart">08.04.2024</enrichment>
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    <enrichment key="date_peer_review">21.10.2024</enrichment>
    <author>Elena Ermilova</author>
    <author>Andreas Hertwig</author>
    <author>Thorsten Döhring</author>
    <author>Eva Stanik</author>
    <author>Vincenzo Cotroneo</author>
    <author>Eugenio Gibertini</author>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>Polydopamine</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>Thin Solid Layers</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>X-ray optics</value>
    </subject>
    <subject>
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      <value>Spectroscopic Ellipsometry</value>
    </subject>
    <collection role="ddc" number="620">Ingenieurwissenschaften und zugeordnete Tätigkeiten</collection>
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  <doc>
    <id>60959</id>
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    <language>eng</language>
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    <title language="eng">Signature of the Adsorbed Layer on the glass transition of thin polymer Films: Broadband Dielectric spectroscopy and related techniques</title>
    <abstract language="eng">In well annealed thin polymer films with non-repulsive polymer/substrate interaction with a substrate an irreversibly adsorbed layer is expected to form. These adsorbed layers have shown a great potential for technological applications [1]. However, the growth kinetics and the molecular mobility of the adsorbed layer is still not fully understood. This concerns also the influence of the adsorbed layer on the thickness dependence of the glass transition temperature of thin films. This is partly due to the difficult accessibility of these layers in thin films. Here, the irreversibly adsorbed layers of semi-rigid mail chain polymers like polycarbonate or polysulfone are revealed by solvent-leaching experiments. First, the growth kinetics of these layers is investigated as a function of annealing time. The film thickness, topography and the quality of the adsorbed layer is controlled by Atomic Force Microscopy (AFM). Secondly, the molecular mobility of the adsorbed layer is investigated by Broadband Dielectric Spectroscopy (BDS). A developed nanostructured capacitor arrangement is employed to measure the layer with a free surface. In addition to the dielectric experiments, spectroscopic Ellipsometry measurements are carried out to estimate the glass transition of the thin films. The thickness dependence of the glass transition of the thin films is correlated with the adsorbed layer [2,3].&#13;
&#13;
Acknowledgments&#13;
D. Hülagü and G. Hidde thanked for the help with the ellipsometry measurements.</abstract>
    <enrichment key="eventName">12. Conference on Broabband Dielectric Spectroscopy and its Application</enrichment>
    <enrichment key="eventPlace">Lisbon, Portugal</enrichment>
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    <author>Hassan Omar</author>
    <author>Andreas Hertwig</author>
    <author>Paulina Szymoniak</author>
    <author>Andreas Schönhals</author>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>Thin films</value>
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    <title language="eng">Meeting the UN Sustainable Development Goals with Mechanochemistry</title>
    <abstract language="eng">Chemistry traditionally relies on reactions in solution, but this method is increasingly problematic due to the scale of chemical processes and their economic and environmental impact. Handling residual chemical waste, including solvents, incurs significant costs and environmental pressure. Conversely, novel chemical approaches are needed to address pressing societal issues such as climate change, energy scarcity, food insecurity, and waste pollution. Mechanochemistry, a sustainable chemistry discipline that uses mechanical action to induce chemical reactivity without bulk solvents, is a hot topic in academic research on sustainable and green chemistry. Given its fundamentally different working principles from solution chemistry, mechanochemistry offers more efficient chemical processes and the opportunity to design new chemical reactions. Mechanochemistry has a profound impact on many urgent issues facing our society and it is now necessary to use mechanochemistry to address them. This Minireview aims to provide a guide for using mechanochemistry to meet the United Nations (UN) Sustainable Development Goals (SDGs), thereby contributing to a prosperous society. Detailed analysis shows that mechanochemistry connects with most UN SDGs and offers more cost‐efficiency than other approaches together with a superior environmental performance.</abstract>
    <parentTitle language="eng">Angewandte Chemie International Edition</parentTitle>
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    <author>Jasna Alić</author>
    <author>Moritz-Caspar Schlegel</author>
    <author>Franziska Emmerling</author>
    <author>Tomislav Stolar</author>
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      <language>eng</language>
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      <value>Mechanochemistry</value>
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    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>SDGs</value>
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