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    <title language="eng">A multi-method study of femtosecond laser modification and ablation of amorphous hydrogenated carbon coatings</title>
    <abstract language="eng">e present a study on femtosecond laser treatment of amorphous hydrogen-containing carbon coatings (a-C:H). The coatings were deposited on silicon wafers by a plasma-assisted chemical vapour deposition (PA-CVD), resulting in two different types of material with distinct properties (referred to as “absorbing” and “semi-transparent” coatings in the following). &#13;
The samples were laser-treated with single fs-laser pulses (800 nm center wavelength, 35 fs pulse duration) in the ablative regime. Through a multi-method approach using topometry, Raman spectroscopy, and spectroscopic imaging ellipsometry, we can identify zones and thresholds of diferent fuence dependent efects and have access to the local dielectric function. &#13;
The two coating materials react signifcantly diferent upon laser treatment. We determined the (non-ablative) modifcation threshold fuence for the absorbing coating as 3.6 × 10−2 Jcm−2 and its ablation threshold as 0.22 Jcm−2. The semi-transparent coating does not show such a low-fuence modifcation but exhibits a characteristic interference-based intra-flm ablation mechanism with two distinguishable ablation thresholds at 0.25 and 0.28 Jcm−2,  respectively. The combination of tailored layer materials and correlative imaging spectroscopic methods delivers new insights into the behaviour of materials when treated with ultrashort-pulse laser radiation</abstract>
    <parentTitle language="eng">Applied Physics A</parentTitle>
    <identifier type="doi">10.1007/s00339-024-07980-z</identifier>
    <identifier type="urn">urn:nbn:de:kobv:b43-617829</identifier>
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We determined the (non-ablative) modification threshold fluence for the absorbing coating as &lt;jats:inline-formula&gt;&lt;jats:alternatives&gt;&lt;jats:tex-math&gt;$$3.6\\times {10}^{-2}$$&lt;\/jats:tex-math&gt;&lt;mml:math xmlns:mml=\"http:\/\/www.w3.org\/1998\/Math\/MathML\"&gt;\n                  &lt;mml:mrow&gt;\n                    &lt;mml:mn&gt;3.6&lt;\/mml:mn&gt;\n                    &lt;mml:mo&gt;\u00d7&lt;\/mml:mo&gt;\n                    &lt;mml:msup&gt;\n                      &lt;mml:mrow&gt;\n                        &lt;mml:mn&gt;10&lt;\/mml:mn&gt;\n                      &lt;\/mml:mrow&gt;\n                      &lt;mml:mrow&gt;\n                        &lt;mml:mo&gt;-&lt;\/mml:mo&gt;\n                        &lt;mml:mn&gt;2&lt;\/mml:mn&gt;\n                      &lt;\/mml:mrow&gt;\n                    &lt;\/mml:msup&gt;\n                  &lt;\/mml:mrow&gt;\n                &lt;\/mml:math&gt;&lt;\/jats:alternatives&gt;&lt;\/jats:inline-formula&gt;\u00a0Jcm&lt;jats:sup&gt;\u22122&lt;\/jats:sup&gt; and its ablation threshold as 0.22\u00a0Jcm&lt;jats:sup&gt;\u22122&lt;\/jats:sup&gt;. 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