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Institute
BTU
The controlled dynamics of liquid drops via generation of specific wetting states on a solid surface is of great interests both in the fundamental and applied sciences. Considering that the wettability is strongly dependent on the surface topography and surface roughness, we investigate – through experiments and theory – the effect of laser-induced periodic surface structures (LIPSS) generated on silicon (100) targets as a control parameter of wetting properties. To obtain structured silicon surfaces with different morphological features, we patterned the surface by irradiation with femtosecond pulses from an amplified Ti:Sapphire laser system (790 nm/100 fs/1 kHz) at a fluence in the range of 0.4–1.2 J/cm2 on a spot with a diameter about of 100 μm. Variation of the applied irradiation dose results in surface modifications with the roughness about of a few tens of nanometers are ranging from regular LIPSS patterns with the lateral period of about 500–700 nm to complex agglomerations of 3-D microstructures with several-μm feature size. The theoretical study on the correlation of wetting properties with the surface topography has been performed within a phase field model. We found an excellent agreement of numerical results with experiments.
Recently, we systematically derived a system of two coupled conservation equations governing a thin liquid layer with a deformable surface composed of two completely miscible components [Phys. Fluids 22, 104102 (2010)]. One equation describes the location of the free surface and the second one the evolution of the mean concentration. This lubrication model was investigated previously in linearized form. The study is now extended to the fully nonlinear case of thin liquid films of a binary mixture (in one and two horizontal spatial dimensions) with and without heat transport. For an initially flat and motionless film heated from below, we analyze the component separation induced by the Soret effect. Nonlinear simulations show that the Soret effect can cause a multitude of interesting behaviors, such as oscillatory patterns and solitonlike structures (localized traveling drops or holes). A stronger component separation induced by stronger Soret effects favors faster-moving localized structures. For isothermal systems, we study the fusion and the mixing of two thin liquid films of different but perfectly miscible liquids. Marangoni-driven forces can cause delayed coalescence, ripple formation, and fingering patterns at the borderline between the two liquid layers. A systematic analysis for ripple pattern formation and finger instabilities at different diffusion constants shows that these phenomena appear more pronounced for lower diffusion in the system.
Drops on cylindrical wires
(2013)
The objective in the present paper is to study binary fluids with phase field modeling coupled with Navier-Stokes equations. An extended free energy is proposed to account for the continuous path from immiscible to miscible states. We consider fluid pairs that are immiscible for temperatures below the critical one (consolute temperature) and miscible above it. Our extended phase field equation permits us to move from the immiscible state (governed by the Cahn-Hilliard equation) to the miscible state (defined by the species diffusion equation). The scaling of interface tension and interface width with the distance to the critical point is highlighted. The whole system is mechanically excited showing Faraday instability of a flat interface. A linear stability analysis is performed for the stable case (interface waves) as well as for the unstable Faraday one. For the latter, a Floquet analysis shows the well-known Arnold's tongues as a function of the consolute temperature and depth layer. Moreover, two-dimensional finite difference simulations have been performed allowing us to model nonlinear flow patterns both in miscible and immiscible phases. Linear theory and nonlinear simulations show interesting results such as the diminishing of the wavelength of Faraday waves or a shift of the critical vibration amplitude when the consolute temperature is approached.