TY - GEN A1 - Zhang, Wei A1 - Wang, Han A1 - Hartmann, Carsten A1 - Weber, Marcus A1 - Schütte, Christof T1 - Applications of the cross-entropy method to importance sampling and optimal control of diffusions T2 - SIAM (Society for Industrial and Applied Mathematics) Y1 - 2014 U6 - https://doi.org/10.1137/14096493X SN - 1095-7197 VL - 36 IS - 6 SP - A2654 EP - A2672 ER - TY - GEN A1 - Wang, Han A1 - Hartmann, Carsten A1 - Schütte, Christof T1 - Linear response theory and optimal control for a molecular system under non-equilibrium conditions T2 - Molecular Physics: An International Journal at the Interface Between Chemistry and Physics Y1 - 2013 U6 - https://doi.org/10.1080/00268976.2013.844370 SN - 1362-3028 VL - 111 IS - 22-23 SP - 3555 EP - 3564 ER - TY - GEN A1 - Wang, Han A1 - Hartmann, Carsten A1 - Schütte, Christof A1 - Delle Site, Luigi T1 - Grand-Canonical-like Molecular-Dynamics Simulations by Using an Adaptive-Resolution Technique T2 - PHYSICAL REVIEW X Y1 - 2013 U6 - https://doi.org/10.1103/PhysRevX.3.011018 SN - 2160-3308 VL - 3 IS - 1 SP - 011018 ER - TY - GEN A1 - Agarwal, Animesh A1 - Zhu, Jinglong A1 - Hartmann, Carsten A1 - Wang, Han A1 - Delle Site, Luigi T1 - Molecular dynamics in a Grand Ensemble: Bergmann-Lebowitz model and adaptive resolution simulation T2 - New Journal of Physics Y1 - 2015 U6 - https://doi.org/10.1088/1367-2630/17/8/083042 SN - 1367-2630 VL - 17 ER - TY - GEN A1 - Han, Liuliu A1 - Xu, Xiandong A1 - Wang, Li A1 - Pyczak, Florian A1 - Zhou, Rui A1 - Liu, Yong T1 - A eutectic high-entropy alloy with good high-temperature strength-plasticity balance T2 - Materials Research Letters Y1 - 2019 SN - 2166-3831 VL - 7 IS - 11 SP - 460 EP - 466 ER - TY - GEN A1 - Li, Siyang A1 - Lok, Tow-Jie A1 - Ngo, Shi-Han A1 - Xue, Yaoting A1 - Miao, Zhikun A1 - Feng, Tao A1 - Wang, Lei A1 - Wong, Jie-Wei A1 - Low, Jiatee A1 - Lim, Kai-Yi A1 - Woon, Min-Rou A1 - Neffe, Axel T. A1 - Wong, Tuck-Whye A1 - Li, Tiefeng A1 - Yang, Xuxu A1 - Yang, Wei T1 - A water-recyclable, robust, and self-healing sugar-based supramolecular network enabled by Maillard-analogous initialization of polymerization T2 - Materials horizons N2 - Crosslinked functional polymers exhibit exceptional mechanical and chemical properties critical for applications spanning biomedical engineering, advanced adhesives, and self-healing materials. However, challenges in recycling, either due to irreversible crosslinks or, in the case of covalent adaptable networks (CANs), limited solid-state plasticity that typically requires catalysts, significantly restrict sustainability. To address these limitations, we present a novel water-mediated polymerization strategy inspired by the radical-generating mechanism of the Maillard reaction, utilizing maltose as both an initiator and a functional side group in a simple, catalyst-free, aqueous reaction with acrylamide (AAm). This mild, one-pot reaction occurs below 100 °C, forming adaptively functionalized supramolecular networks (AFSNs) that form supramolecular networks through hydrogen bonding and display dynamic imine linkages to the maltose side chains supporting self-healing and re-shaping. These elastomers are characterized by impressive mechanical strength (up to 5 MPa tensile strength), high elongation (up to 1000%), notable fracture energy (36 kJ m−2), robust adhesive performance (up to 4.8 MPa), and rapid self-healing capability at room temperature. Crucially, the elastomer's supramolecular network can be fully and repeatedly dissolved and reprocessed using only water, preserving mechanical integrity without chemical degradation. This sustainable approach provides a practical solution for synthesizing and recycling high-performance crosslinked materials while eliminating environmental hazards, guiding the future development of green polymer chemistry and functional material design. KW - Recycling KW - biobased polymer KW - self-healing KW - Maillard Y1 - 2026 U6 - https://doi.org/10.1039/D5MH01828E SN - 2051-6347 VL - 13 IS - 1 SP - 219 EP - 232 PB - Royal Society of Chemistry (RSC) CY - Cambridge ER -