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    <title language="eng">Unraveling van der Waals epitaxy: A real-time in-situ study of MoSe2 growth on graphene/Ru(0001)</title>
    <abstract language="eng">In the present work we investigate the growth of monolayer MoSe2 on selenium-intercalated graphene on Ru(0001), a model layered heterostructure combining a transition metal dichalcogenide with graphene, using low energy electron microscopy and micro-diffraction. Real-time observation of MoSe2 on graphene growth reveals the island nucleation dynamics at the nanoscale. Upon annealing, larger islands are formed by sliding and attachment of multiple nanometer-sized MoSe2 flakes. Local micro-spot angle-resolved photoemission spectroscopy reveals the electronic structure of the heterostructure, indicating that no charge transfer occurs within adjacent layers. The observed behavior is attributed to intercalation of Se at the graphene/Ru(0001) interface. The unperturbed nature of the proposed heterostructure therefore renders it as a model system for investigations of graphene supported TMD nanostructures.</abstract>
    <parentTitle language="eng">Ultramicroscopy</parentTitle>
    <identifier type="issn">0304-3991</identifier>
    <identifier type="issn">1879-2723</identifier>
    <identifier type="doi">10.1016/j.ultramic.2023.113749</identifier>
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    <author>
      <firstName>Lars</firstName>
      <lastName>Buß</lastName>
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    <submitter>
      <firstName>Karsten</firstName>
      <lastName>Henkel</lastName>
    </submitter>
    <author>
      <firstName>Nicolas</firstName>
      <lastName>Braud</lastName>
    </author>
    <author>
      <firstName>Moritz</firstName>
      <lastName>Ewert</lastName>
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    <author>
      <firstName>Matteo</firstName>
      <lastName>Jugovac</lastName>
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    <author>
      <firstName>Tevfik Onur</firstName>
      <lastName>Menteş</lastName>
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    <author>
      <firstName>Andrea</firstName>
      <lastName>Locatelli</lastName>
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      <firstName>Jens</firstName>
      <lastName>Falta</lastName>
    </author>
    <author>
      <firstName>Jan Ingo</firstName>
      <lastName>Flege</lastName>
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    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>Graphene</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>transition metal dichalcogenides (TMDs)</value>
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    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>angle-resolved photoemission spectroscopy (ARPES)</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>Heterostructures</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>low  energy electron microscopy (LEEM)</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>low  energy electron diffraction (LEED)</value>
    </subject>
    <collection role="institutes" number="1503">FG Angewandte Physik und Halbleiterspektroskopie</collection>
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    <issue>19</issue>
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    <title language="eng">Rubidium intercalation in epitaxial monolayer graphene</title>
    <abstract language="eng">Alkali metal intercalation of graphene layers has been of particular interest due to potential applications in electronics, energy storage, and catalysis. Rubidium (Rb) is one of the largest alkali metals and among the least investigated as an intercalant. Here, we report a systematic investigation, with a multi-technique approach, of the phase formation of Rb under epitaxial monolayer graphene on SiC(0001). We explore a wide phase space with two control parameters: the Rb density (i.e., deposition time) and sample temperature (i.e., room and low temperature). We reveal the emergence of (2 × 2) and [sqrt(3) x (sqrt3)] R30° structures formed by a single alkali metal layer intercalated between monolayer graphene and the interfacial C-rich reconstructed surface, also known as the buffer layer. Rb intercalation also results in strong n-type doping of the graphene layer. Upon progressively annealing to higher temperatures, we first reveal the diffusion of Rb atoms, which results in the enlargement of intercalated areas. As desorption sets in, intercalated regions progressively shrink and fragment. Eventually, at approximately 600 °C, the initial surface is retrieved, indicating the reversibility of the intercalation process.</abstract>
    <parentTitle language="eng">Nanoscale</parentTitle>
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    </author>
    <author>
      <firstName>Stefan</firstName>
      <lastName>Heun</lastName>
    </author>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>Graphene</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>N-type doping</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>Micro-spot low-energy electron diffraction (µLEED)</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>Scanning tunneling microscopy (STM)</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>Low-energy electron microscopy (LEEM)</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>Density functional theory (DFT)</value>
    </subject>
    <collection role="institutes" number="1503">FG Angewandte Physik und Halbleiterspektroskopie</collection>
  </doc>
</export-example>
