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    <title language="eng">Multifunctional Roles of Iron Oxide Nanoparticles in a Reversible Shape‐Memory Composite</title>
    <abstract language="eng">The utilization of functional fillers in the development of composite materials has come a long way since its advent to improve physical, chemical, or mechanical properties of the base material. However, the heterogenous roles contributed by a single type of filler remain uncommon in this field. Here the endowment of various modifications to a 1,8‐octanediol/1,12‐dodecanedioic acid/citric acid (OD/DDA/CA) matrix through the incorporation of iron oxide nanoparticles (IONPs) is reported. Owing to the relaxation and hysteresis loss behaviors of IONPs when exposed to an alternating magnetic field (AMF), the composites demonstrate a magnetothermal response. Similarly, the excitation and relaxation of electrons in IONPs under near‐infrared light (NIR) enable photothermic‐responsiveness. In combination, two findings nurtured an observed shape‐memory effect when the samples are under actuation by these indirect stimuli, where a shape recovery ratio (≥98%) and reversible strain (≤7%) are recorded. Moreover, the catalytic role of IONPs aided transesterification in the covalent network, demonstrated by successful repeated cycles of shape reconfiguration of the samples. This work highlights the prospectives of multifunctional composite fillers in the exploration of bio‐derived composite smart materials.</abstract>
    <parentTitle language="eng">Advanced Functional Materials</parentTitle>
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However, the heterogenous roles contributed by a single type of filler remain uncommon in this field. Here the endowment of various modifications to a 1,8\u2010octanediol\/1,12\u2010dodecanedioic acid\/citric acid (OD\/DDA\/CA) matrix through the incorporation of iron oxide nanoparticles (IONPs) is reported. Owing to the relaxation and hysteresis loss behaviors of IONPs when exposed to an alternating magnetic field (AMF), the composites demonstrate a magnetothermal response. Similarly, the excitation and relaxation of electrons in IONPs under near\u2010infrared light (NIR) enable photothermic\u2010responsiveness. In combination, two findings nurtured an observed shape\u2010memory effect when the samples are under actuation by these indirect stimuli, where a shape recovery ratio (\u226598%) and reversible strain (\u22647%) are recorded. 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    <author>
      <firstName>Mun‐Oon</firstName>
      <lastName>Fong</lastName>
    </author>
    <submitter>
      <firstName>Axel T.</firstName>
      <lastName>Neffe</lastName>
    </submitter>
    <author>
      <firstName>Xiangping</firstName>
      <lastName>Chen</lastName>
    </author>
    <author>
      <firstName>Jie‐Wei</firstName>
      <lastName>Wong</lastName>
    </author>
    <author>
      <firstName>Tow‐Jie</firstName>
      <lastName>Lok</lastName>
    </author>
    <author>
      <firstName>Siyang</firstName>
      <lastName>Li</lastName>
    </author>
    <author>
      <firstName>Jia Tee</firstName>
      <lastName>Low</lastName>
    </author>
    <author>
      <firstName>Nur Syahirra</firstName>
      <lastName>Nordin</lastName>
    </author>
    <author>
      <firstName>Zhikun</firstName>
      <lastName>Miao</lastName>
    </author>
    <author>
      <firstName>Qiannan</firstName>
      <lastName>Hu</lastName>
    </author>
    <author>
      <firstName>Axel T.</firstName>
      <lastName>Neffe</lastName>
    </author>
    <author>
      <firstName>Tuck‐Whye</firstName>
      <lastName>Wong</lastName>
    </author>
    <author>
      <firstName>Tiefeng</firstName>
      <lastName>Li</lastName>
    </author>
    <author>
      <firstName>Wei</firstName>
      <lastName>Yang</lastName>
    </author>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>Shape-Memory Polymer</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>Composite</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>Iron Oxide Nanoparticle</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>bio-based</value>
    </subject>
    <collection role="institutes" number="2203">FG Organische Chemie mit dem Schwerpunkt Polymere</collection>
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    <pageNumber/>
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    <issue>1</issue>
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    <type>article</type>
    <publisherName>Informa UK Limited</publisherName>
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    <title language="eng">Recent Advances in the Field of Shape-Memory Polymer from Bio-Based Precursors: Review and Perspective</title>
    <abstract language="eng">Shape-memory polymers (SMPs) are predominantly derived from nonrenewable resources due to their low production cost, wide availability, and refined techniques for processing and tailoring SMP properties. However, the heavy reliance on these nonrenewable resources poses significant concerns regarding resource depletion and the long-term sustainability of the technology. As petroleum-based resources, which have traditionally fueled the polymer industry, become increasingly scarce, it is imperative to develop bio-based SMPs. This shift is essential not just for resource conservation but to ensure the continued viability and sustainability of SMP technology in the face of dwindling petroleum supplies. This review provides an overview of bio-based SMPs, which are synthesized from renewable precursors or through chemical variation and functionalization of biopolymers. The molecular mechanism and design strategy for the shape-memory effect (SME), syntheses, unique characteristics and shape-memory performance for these bio-based SMPs are covered. Furthermore, this review highlights novel insights and proposes promising directions for the development of sustainable SMPs with comparable performance to their nonrenewable counterparts. By focusing on bio-based alternatives, this work aims to motivate the exploration and advancement of next-generation sustainable SMPs.</abstract>
    <parentTitle language="eng">Polymer Reviews</parentTitle>
    <identifier type="doi">10.1080/15583724.2024.2427827</identifier>
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      <firstName>Farah Hidayah</firstName>
      <lastName>Jamaludin</lastName>
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      <lastName>Neffe</lastName>
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      <firstName>Nur Syahirra</firstName>
      <lastName>Nordin</lastName>
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      <firstName>Xinge</firstName>
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      <firstName>Jie‐Wei</firstName>
      <lastName>Wong</lastName>
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      <firstName>Zhixian</firstName>
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      <firstName>Chunxin</firstName>
      <lastName>Ma</lastName>
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      <firstName>Qian</firstName>
      <lastName>Zhao</lastName>
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      <firstName>Tuck‐Whye</firstName>
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      <firstName>Axel T.</firstName>
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      <firstName>Tiefeng</firstName>
      <lastName>Li</lastName>
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    <title language="eng">A water-recyclable, robust, and self-healing sugar-based supramolecular network enabled by Maillard-analogous initialization of polymerization</title>
    <abstract language="eng">Crosslinked functional polymers exhibit exceptional mechanical and chemical properties critical for applications spanning biomedical engineering, advanced adhesives, and self-healing materials. However, challenges in recycling, either due to irreversible crosslinks or, in the case of covalent adaptable networks (CANs), limited solid-state plasticity that typically requires catalysts, significantly restrict sustainability. To address these limitations, we present a novel water-mediated polymerization strategy inspired by the radical-generating mechanism of the Maillard reaction, utilizing maltose as both an initiator and a functional side group in a simple, catalyst-free, aqueous reaction with acrylamide (AAm). This mild, one-pot reaction occurs below 100 °C, forming adaptively functionalized supramolecular networks (AFSNs) that form supramolecular networks through hydrogen bonding and display dynamic imine linkages to the maltose side chains supporting self-healing and re-shaping. These elastomers are characterized by impressive mechanical strength (up to 5 MPa tensile strength), high elongation (up to 1000%), notable fracture energy (36 kJ m−2), robust adhesive performance (up to 4.8 MPa), and rapid self-healing capability at room temperature. Crucially, the elastomer's supramolecular network can be fully and repeatedly dissolved and reprocessed using only water, preserving mechanical integrity without chemical degradation. This sustainable approach provides a practical solution for synthesizing and recycling high-performance crosslinked materials while eliminating environmental hazards, guiding the future development of green polymer chemistry and functional material design.</abstract>
    <parentTitle language="eng">Materials horizons</parentTitle>
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