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  <doc>
    <id>28969</id>
    <completedYear/>
    <publishedYear>2022</publishedYear>
    <thesisYearAccepted/>
    <language>eng</language>
    <pageFirst/>
    <pageLast/>
    <pageNumber>8</pageNumber>
    <edition/>
    <issue>17</issue>
    <volume>9</volume>
    <type>articler</type>
    <publisherName/>
    <publisherPlace/>
    <creatingCorporation/>
    <contributingCorporation/>
    <belongsToBibliography>0</belongsToBibliography>
    <completedDate>2022-06-15</completedDate>
    <publishedDate>--</publishedDate>
    <thesisDateAccepted>--</thesisDateAccepted>
    <title language="eng">Atomic Layer Engineering of Aluminum-Doped Zinc Oxide films for Efficient and Stable Perovskite Solar Cells</title>
    <abstract language="eng">Atomic layer deposition (ALD) has been considered as an efficient method to deposit high quality and uniform thin films of various electron transport materials for perovskite solar cells (PSCs). Here, the effect of deposition sequence in the ALD process of aluminum-doped zinc oxide (AZO) films on the performance and stability of PSCs is investigated. Particularly, the surface of AZO film is terminated by diethylzinc (DEZ)/H2O (AZO-1) or trimethylaluminum (TMA)/H2O pulse (AZO-2), and investigated with surface-sensitive X-ray photoelectron spectroscopy technique. It is observed that AZO-2 significantly enhances the thermal stability of the upcoming methylammonium lead iodide (MAPbI3) layer and facilitates charge transport at the interface as evidenced by photoluminescence spectroscopes and favorable interfacial band alignment. Finally, planar-type PSC with AZO-2 layer exhibits a champion power conversion efficiency of 18.09% with negligible hysteresis and retains 82% of the initial efficiency after aging for 100 h under ambient conditions (relative humidity 40 ± 5%). These results highlight the importance of atomic layer engineering for developing efficient and stable PSCs.</abstract>
    <parentTitle language="eng">Advanced Materials Interfaces</parentTitle>
    <identifier type="issn">2196-7350</identifier>
    <identifier type="doi">10.1002/admi.202200575</identifier>
    <enrichment key="BTU">an der BTU erstellt / created at BTU</enrichment>
    <enrichment key="Artikelnummer">2200575</enrichment>
    <enrichment key="opus.source">publish</enrichment>
    <enrichment key="opus.doi.autoCreate">false</enrichment>
    <enrichment key="opus.urn.autoCreate">false</enrichment>
    <enrichment key="Fprofil">1 Energiewende und Dekarbonisierung / Energy Transition and Decarbonisation</enrichment>
    <enrichment key="Fprofil">4 Künstliche Intelligenz und Sensorik / Artificial Intelligence and Sensor Technology</enrichment>
    <author>
      <firstName>Joanna</firstName>
      <lastName>Kruszyńska</lastName>
    </author>
    <submitter>
      <firstName>Karsten</firstName>
      <lastName>Henkel</lastName>
    </submitter>
    <author>
      <firstName>Jakub</firstName>
      <lastName>Ostapko</lastName>
    </author>
    <author>
      <firstName>Veysel</firstName>
      <lastName>Ozkaya</lastName>
    </author>
    <author>
      <firstName>Belkis</firstName>
      <lastName>Surucu</lastName>
    </author>
    <author>
      <firstName>Oliwia</firstName>
      <lastName>Szawcow</lastName>
    </author>
    <author>
      <firstName>Kostiantyn</firstName>
      <lastName>Nikiforow</lastName>
    </author>
    <author>
      <firstName>Marcin</firstName>
      <lastName>Hołdyński</lastName>
    </author>
    <author>
      <firstName>Mohammad Mahdi</firstName>
      <lastName>Tavakoli</lastName>
    </author>
    <author>
      <firstName>Pankaj</firstName>
      <lastName>Yadav</lastName>
    </author>
    <author>
      <firstName>Małgorzata</firstName>
      <lastName>Kot</lastName>
    </author>
    <author>
      <firstName>Grzegorz Piotr</firstName>
      <lastName>Kołodziej</lastName>
    </author>
    <author>
      <firstName>Mateusz</firstName>
      <lastName>Wlazło</lastName>
    </author>
    <author>
      <firstName>Soumitra</firstName>
      <lastName>Satapathi</lastName>
    </author>
    <author>
      <firstName>Seckin</firstName>
      <lastName>Akin</lastName>
    </author>
    <author>
      <firstName>Daniel</firstName>
      <lastName>Prochowicz</lastName>
    </author>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>atomic layer deposition</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>electron transporting layers</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>perovskites</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>solar cells</value>
    </subject>
    <subject>
      <language>eng</language>
      <type>uncontrolled</type>
      <value>stability of perovskite solar cells</value>
    </subject>
    <collection role="institutes" number="1503">FG Angewandte Physik und Halbleiterspektroskopie</collection>
  </doc>
</export-example>
