@misc{SeiboldArpaiaYingYingetal., author = {Seibold, G{\"o}tz and Arpaia, Riccardo and Ying Ying, Peng and Fumagalli, Roberto and Braicovich, Lucio and Di Castro, Carlo and Grilli, Marco and Ghiringhelli, Giacomo Claudio and Caprara, Sergio}, title = {Strange metal behaviour from charge density fluctuations in cuprates}, series = {Communications Physics}, volume = {4}, journal = {Communications Physics}, issn = {2399-3650}, doi = {10.1038/s42005-020-00505-z}, pages = {1 -- 6}, abstract = {Besides the mechanism responsible for high critical temperature superconductivity, the grand unresolved issue of the cuprates is the occurrence of a strange metallic state above the so-called pseudogap temperature T*. Even though such state has been successfully described within a phenomenological scheme, the so-called Marginal Fermi-Liquid theory, a microscopic explanation is still missing. However, recent resonant X-ray scattering experiments identified a new class of charge density fluctuations characterized by low characteristic energies and short correlation lengths, which are related to the well-known charge density waves. These fluctuations are present over a wide region of the temperature-vs-doping phase diagram and extend well above T*. Here we investigate the consequences of charge density fluctuations on the electron and transport properties and find that they can explain the strange metal phenomenology. Therefore, charge density fluctuations are likely the long-sought microscopic mechanism underlying the peculiarities of the metallic state of cuprates.}, language = {en} } @misc{WahlbergArpaiaSeiboldetal., author = {Wahlberg, Eric and Arpaia, Riccardo and Seibold, G{\"o}tz and Rossi, Matteo and Fumagalli, Roberto and Trabaldo, Edoardo and Brookes, Nicholas B. and Braicovich, Lucio and Caprara, Sergio and Lombardi, Floriana and Gran, Ulf and Ghiringhelli, Giacomo Claudio and Bauch, Thilo}, title = {Restored strange metal phase through suppression of charge density waves in underdoped YBa2Cu3O7-δ}, series = {Science}, volume = {373}, journal = {Science}, number = {6562}, doi = {10.1126/science.abc8372}, pages = {1506 -- 1510}, abstract = {The normal state of optimally doped cuprates is dominated by the "strange metal" phase that shows a linear temperature (T) dependence of the resistivity persisting down to the lowest T. For underdoped cuprates, this behavior is lost below the pseudogap temperature T*, where charge density waves (CDWs), together with other intertwined local orders, characterize the ground state. We found that the T-linear resistivity of highly strained, ultrathin, underdoped YBa2Cu3O7-δ films is restored when the CDW amplitude, detected by resonant inelastic x-ray scattering, is suppressed. This observation suggests an intimate connection between the onset of CDWs and the departure from T-linear resistivity in underdoped cuprates. Our results illustrate the potential of using strain control to manipulate the ground state of quantum materials.}, language = {en} } @misc{MirarchiArpaiaWahlbergetal., author = {Mirarchi, Giovanni and Arpaia, Riccardo and Wahlberg, Eric and Bauch, Thilo and Kalaboukhov, Alexei and Caprara, Sergio and Di Castro, Carlo and Grilli, Marco and Lombardi, Floriana and Seibold, G{\"o}tz}, title = {Tuning the ground state of cuprate superconducting thin films by nanofaceted substrates}, series = {Communications Materials}, journal = {Communications Materials}, number = {5}, doi = {10.1038/s43246-024-00582-5}, pages = {1 -- 6}, abstract = {Anisotropic transport properties have been assessed in a number of cuprate superconductors, providing evidence for a nematic state. We have recently shown that in ultra-thin YBa2Cu3O7-δ films, where nematicity is induced via strain engineering, there is a suppression of charge density wave scattering along the orthorhombic a-axis and a concomitant enhancement of strange metal behavior along the b-axis. Here we develop a microscopic model, that is based on the strong interaction between the substrate facets and the thin film, to account for the unconventional phenomenology. Based on the atomic force microscopy imaging of the substrates' surface, the model is able to predict the absence (presence) of nematicity and the resulting transport properties in films grown on SrTiO3 (MgO) substrates. Our result paves the way to new tuning capabilities of the ground state of high-temperature superconductors by substrate engineering.}, language = {en} } @misc{WahlbergArpaiaChakrabortyetal., author = {Wahlberg, Eric and Arpaia, Riccardo and Chakraborty, Debmalya and Kalaboukhov, Alexei and Vignolles, David and Proust, Cyril and Black-Schaffer, Annica M. and Bauch, Thilo and Seibold, G{\"o}tz and Lombardi, Floriana}, title = {Boosting superconductivity in ultrathin YBa₂Cu₃O₇-δ films via nanofaceted substrates}, series = {Nature communications}, volume = {17}, journal = {Nature communications}, publisher = {Springer Nature}, address = {London}, issn = {2041-1723}, doi = {10.1038/s41467-025-67500-2}, pages = {1 -- 8}, abstract = {In cuprate high-temperature superconductors the doping level is fixed during synthesis, hence the charge carrier density per CuO2 plane cannot be easily tuned by conventional gating, unlike in 2D materials. Strain engineering has recently emerged as a powerful tuning knob for manipulating the properties of cuprates, in particular charge and spin orders, and their delicate interplay with superconductivity. In thin films, additional tunability can be introduced by the substrate surface morphology, particularly nanofacets formed by substrate surface reconstruction. Here we show a remarkable enhancement of the superconducting onset temperature and the upper critical magnetic field Hc,2 in nanometer-thin YBa2Cu3O7-δ films grown on a substrate with a nanofaceted surface. We theoretically show that the enhancement is driven by electronic nematicity and unidirectional charge density waves, where both elements are captured by an additional effective potential at the interface between the film and the uniquely textured substrate. Our findings show a new paradigm in which substrate engineering can effectively enhance the superconducting properties of cuprates. This approach opens an exciting frontier in the design and optimization of high-performance superconducting materials.}, language = {en} }